Atmospheric & Oceanic Science

Permanent URI for this communityhttp://hdl.handle.net/1903/2264

Formerly known as the Department of Meteorology.

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A 20-YEAR CLIMATOLOGY OF GLOBAL ATMOSPHERIC METHANE FROM HYPERSPECTRAL THERMAL INFRARED SOUNDERS WITH SOME APPLICATIONS
(2022) Zhou, Lihang; Warner, Juying; Atmospheric and Oceanic Sciences; Digital Repository at the University of Maryland; University of Maryland (College Park, Md.)
Atmospheric Methane (CH4) is the second most important greenhouse gas after carbon dioxide (CO2), and accounts for approximately 20% of the global warming produced by all well-mixed greenhouse gases. Thus, its spatiotemporal distributions and relevant long-term trends are critical to understanding the sources, sinks, and global budget of atmospheric composition, as well as the associated climate impacts. The current suite of hyperspectral thermal infrared sounders has provided continuous global methane data records since 2002, starting with the Atmospheric Infrared Sounder (AIRS) onboard the NASA EOS/Aqua satellite launched on 2 May 2002. The Cross-track Infrared Sounder (CrIS) was launched onboard the Suomi National Polar Orbiting Partnership (SNPP) on 28 October 2011 and then on NOAA-20 on 18 November 2017. The Infrared Atmospheric Sounding Interferometer (IASI) was launched onboard the EUMETSAT MetOp-A on 19 October 2006, followed by MetOp-B on 17 September 2012, then Metop-C on 7 November 2018. In this study, nearly two decades of global CH4 concentrations retrieved from the AIRS and CrIS sensors were analyzed. Results indicate that the global mid-upper tropospheric CH4 concentrations (centered around 400 hPa) increased significantly from 2003 to 2020, i.e., with an annual average of ~1754 ppbv in 2003 and ~1839 ppbv in 2020. The total increase is approximately 85 ppbv representing a +4.8% change in 18 years. More importantly, the rate of increase was derived using satellite measurements and shown to be consistent with the rate of increase previously reported only from in-situ observational measurements. It further confirmed that there was a steady increase starting in 2007 that became stronger since 2014, as also reported from the in-situ observations. In addition, comparisons of the methane retrieved from the AIRS and CrIS against in situ measurements from NOAA Global Monitoring Laboratory (GML) were conducted. One of the key findings of this comparative study is that there are phase shifts in the seasonal cycles between satellite thermal infrared measurements and ground measurements, especially in the middle to high latitudes in the northern hemisphere. Through this, an issue common in the hyperspectral thermal sensor retrievals were discovered that was unknown previously and offered potential solutions. We also conducted research on some applications of the retrieval products in monitoring the changes of CH4 over the selected regions (the Arctic and South America). Detailed analyses based on local geographic changes related to CH4 concentration increases were discussed. The results of this study concluded that while the atmospheric CH4 concentration over the Arctic region has been increasing since the early 2000s, there were no catastrophic sudden jumps during the period of 2008-2012, as indicated by the earlier studies using pre-validated retrieval products. From our study of CH4 climatology using hyperspectral infrared sounders, it has been proved that the CH4 from hyperspectral sounders provide valuable information on CH4 for the mid-upper troposphere and lower stratosphere. Future approaches are suggested that include: 1) Utilizing extended data records for CH4 monitoring using AIRS, CrIS, and other potential new generation hyperspectral infrared sensors; 2). Improving the algorithms for trace gas retrievals; and 3). Enhancing the capacity to detect CH4 changes and anomalies with radiance signals from hyperspectral infrared sounders.
A 7-Year Climatology of Warm-Sector Heavy Rainfall over South China during the Pre-Summer Months
(MDPI, 2021-07-15) Chen, Tao; Zhang, Da-Lin
In view of the limited predictability of heavy rainfall (HR) events and the limited understanding of the physical mechanisms governing the initiation and organization of the associated mesoscale convective systems (MCSs), a composite analysis of 58 HR events over the warm sector (i.e., far ahead of the surface cold front), referred to as WSHR events, over South China during the months of April to June 2008~2014 is performed in terms of precipitation, large-scale circulations, pre-storm environmental conditions, and MCS types. Results show that the large-scale circulations of the WSHR events can be categorized into pre-frontal, southwesterly warm and moist ascending airflow, and low-level vortex types, with higher frequency occurrences of the former two types. Their pre-storm environments are characterized by a deep moist layer with >50 mm column-integrated precipitable water, high convective available potential energy with the equivalent potential temperature of ≥340 K at 850 hPa, weak vertical wind shear below 400 hPa, and a low-level jet near 925 hPa with weak warm advection, based on atmospheric parameter composite. Three classes of the corresponding MCSs, exhibiting peak convective activity in the afternoon and the early morning hours, can be identified as linear-shaped, a leading convective line adjoined with trailing stratiform rainfall, and comma-shaped, respectively. It is found that many linear-shaped MCSs in coastal regions are triggered by local topography, enhanced by sea breezes, whereas the latter two classes of MCSs experience isentropic lifting in the southwesterly warm and moist flows. They all develop in large-scale environments with favorable quasi-geostrophic forcing, albeit weak. Conceptual models are finally developed to facilitate our understanding and prediction of the WSHR events over South China.
A Century of Observed Temperature Change in the Indian Ocean
(Wiley, 2022-06-25) Wenegrat, J. O.; Bonanno, E.; Rack, U.; Gebbie, G.
The Indian Ocean is warming rapidly, with widespread effects on regional weather and global climate. Sea-surface temperature records indicate this warming trend extends back to the beginning of the 20th century, however the lack of a similarly long instrumental record of interior ocean temperatures leaves uncertainty around the subsurface trends. Here we utilize unique temperature observations from three historical German oceanographic expeditions of the late 19th and early 20th centuries: SMS Gazelle (1874–1876), Valdivia (1898–1899), and SMS Planet (1906–1907). These observations reveal a mean 20th century ocean warming that extends over the upper 750 m, and a spatial pattern of subsurface warming and cooling consistent with a 1°–2° southward shift of the southern subtropical gyre. These interior changes occurred largely over the last half of the 20th century, providing observational evidence for the acceleration of a multidecadal trend in subsurface Indian Ocean temperature.
A CloudSat and CALIPSO-based evaluation of the effects of thermodynamic instability and aerosol loading on Amazon Basin deep convection and lightning
(2023-08-14) Allen, Dale
The Amazon Basin, which plays an important role in the carbon and water cycle, is under stress due to changes in climate, agricultural practices, and deforestation. The Basin includes a rainforest in the northwest and a mix of deforested areas, savannah-type vegetation, and agriculture in the southeast. The effects of instability and aerosol loading on thunderstorms in the Basin (75-45° W, 0-15° S) were examined during mid-August through mid-December, a period with large variations in aerosols, intense convective storms, and plentiful flashes. The analysis used measurements of radar reflectivity, ice water content (IWC), and aerosol type from instruments aboard the CloudSat and CALIPSO satellites, flash rates from the ground-based STARNET network, and aerosol optical depth (AOD) from a surface network and a meteorological re-analysis. After controlling for convective available potential energy (CAPE), a measure of instability, it was found that thunderstorms that developed under dirty (high-AOD) conditions were approximately 1.5 km deeper, had 50% more IWC, and more than two times as many flashes as storms that developed under clean (low-AOD) conditions. Flash rates were also found to be larger during periods when smoke rather than dust was common in the lower troposphere, likely because these periods were less stable.
A Neural-Network Based MPAS—Shallow Water Model and Its 4D-Var Data Assimilation System
(MDPI, 2023-01-10) Tian, Xiaoxu; Conibear, Luke; Steward, Jeffrey
The technique of machine learning has been increasingly applied in numerical weather predictions. The aim of this study is to explore the application of a neural network in data assimilation by making use of the convenience in obtaining the tangent linear and adjoint (TL/AD) of a neural network (NN) and formulating a NN-based four-dimensional variational (4D-Var) DA system. A NN-based shallow water (SW) model is developed in this study. The NN model consists of three layers. The weights and biases in the NN-based SW model are trained with 60 years of hourly ERA5 geopotentials and wind field at 500 hPa as initial conditions and the corresponding 12-h forecasts by Model for Prediction Across Scales (MPAS)-SW, in total of 534,697 sets of samples. The 12-h forecasts from independent dates made by NN-based SW prove to closely emulate the simulations by the actual MPAS-SW model. This study further shows that the TL/AD of an NN model can be easily developed and validated. The ease of obtaining the TL/AD makes NN conveniently applicable in various aspects within a data assimilation (DA) system. To demonstrate such, a continuous 4D-Var DA system is also developed with the forward NN and its adjoint. To demonstrate the functionality of the NN-based 4D-Var DA system, the results from a higher resolution simulation will be treated as observations and assimilated to analyze the low resolution initial conditions. The forecasts starting from the analyzed initial conditions will be compared with those without assimilation to demonstrate improvements.
A Study of the Oklahoma City Urban Heat Island Effect Using a WRF/Single-Layer Urban Canopy Model, a Joint Urban 2003 Field Campaign, and MODIS Satellite Observations
(MDPI, 2017-09-07) Zhang, Hengyue; Jin, Menglin S.; Leach, Martin
The urban heat island effect (UHI) for inner land regions was investigated using satellite data, ground observations, and simulations with an Single-Layer Urban Canopy Parameterization (SLUCP) coupled into the regional Weather Research Forecasting model (WRF, http://wrf-model.org/index.php). Specifically, using the satellite-observed surface skin temperatures (Tskin), the intensity of the UHI was first compared for two inland cities (Xi’an City, China, and Oklahoma City (OKC)), which have different city populations and building densities. The larger population density and larger building density in Xi’an lead to a stronger skin-level UHI by 2 °C. However, the ground observed 2 m surface air temperature (Tair) observations showed an urban cooling island effect (UCI) over the downtown region in OKC during the daytime of 19 July 2003, from a DOE field campaign (Joint Urban 2003). To understand this contrast between satellite-based Tskin and ground-based Tair, a sensitivity study using WRF/SLUCP was analyzed. The model reproduced a UCI in OKC. Furthermore, WRF/Noah/SLUCM simulations were also compared with the Joint Urban 2003 ground observations, including wind speeds, wind directions, and energy fluxes. Although the WRF/SLUCM model failed to simulate these variables accurately, it reproduced the diurnal variations of surface temperatures, wind speeds, wind directions, and energy fluxes reasonably well.
ADVANCES IN SEQUENTIAL DATA ASSIMILATION AND NUMERICAL WEATHER FORECASTING: AN ENSEMBLE TRANSFORM KALMAN-BUCY FILTER, A STUDY ON CLUSTERING IN DETERMINISTIC ENSEMBLE SQUARE ROOT FILTERS, AND A TEST OF A NEW TIME STEPPING SCHEME IN AN ATMOSPHERIC MODEL
(2012) Amezcua, Javier; Kalnay, Eugenia; Ide, Kayo; Atmospheric and Oceanic Sciences; Digital Repository at the University of Maryland; University of Maryland (College Park, Md.)
This dissertation deals with aspects of sequential data assimilation (in particular ensemble Kalman filtering) and numerical weather forecasting. In the first part, the recently formulated Ensemble Kalman-Bucy (EnKBF) filter is revisited. It is shown that the previously used numerical integration scheme fails when the magnitude of the background error covariance grows beyond that of the observational error covariance in the forecast window. Therefore, we present a suitable integration scheme that handles the stiffening of the differential equations involved and doesn't represent further computational expense. Moreover, a transform-based alternative to the EnKBF is developed: under this scheme, the operations are performed in the ensemble space instead of in the state space. Advantages of this formulation are explained. For the first time, the EnKBF is implemented in an atmospheric model. The second part of this work deals with ensemble clustering, a phenomenon that arises when performing data assimilation using of deterministic ensemble square root filters in highly nonlinear forecast models. Namely, an M-member ensemble detaches into an outlier and a cluster of M-1 members. Previous works may suggest that this issue represents a failure of EnSRFs; this work dispels that notion. It is shown that ensemble clustering can be reverted also due to nonlinear processes, in particular the alternation between nonlinear expansion and compression of the ensemble for different regions of the attractor. Some EnSRFs that use random rotations have been developed to overcome this issue; these formulations are analyzed and their advantages and disadvantages with respect to common EnSRFs are discussed. The third and last part contains the implementation of the Robert-Asselin-Williams (RAW) filter in an atmospheric model. The RAW filter is an improvement to the widely popular Robert-Asselin filter that successfully suppresses spurious computational waves while avoiding any distortion in the mean value of the function. Using statistical significance tests both at the local and field level, it is shown that the climatology of the SPEEDY model is not modified by the changed time stepping scheme; hence, no retuning of the parameterizations is required. It is found the accuracy of the medium-term forecasts is increased by using the RAW filter.
Air Pollutant Concentrations and Trends over the Eastern U.S. and China: Aircraft Measurements and Numerical Simulations
(2012) He, Hao; Dickerson, Russell R.; Atmospheric and Oceanic Sciences; Digital Repository at the University of Maryland; University of Maryland (College Park, Md.)
In the last several decades, efforts have been made to mitigate air pollution all around the world. With surface observations showing substantial decrease of criteria pollutants, including O3, NOx, CO and SO2, the long-term aircraft measurements over the eastern U.S. provide a unique opportunity to study the trend of the air pollutant column contents and the regional transport in the free troposphere. Analyses of the historical data indicated ~2.0 Dobson Unit/decade decrease in tropospheric O3 columns over the eastern U.S. with a similar decreasing trend of CO. The statistical analysis also showed a significant decreasing trend for tropospheric SO2. Analyses of the EPA CEMS emission data showed parallel reductions. A case study of tropospheric O3 and SO2 over downwind area of Baltimore showed that the regional transport by westerly wind from Ohio and Pennsylvania play an important role in the local air quality issues. As the second largest economy in the world, China's rapid economic growth in the last decade lead to a dramatic increase in energy demand, which relied heavily on coal burning. The enormous amount of SO2 emissions caused severe environmental issues including acid deposition and particulate matter pollution. To mitigate these air quality problems, strict control measures and regulations were applied to abate sulfur emissions, especially before and during the 2008 Beijing Olympics. Aircraft measurements of tropospheric SO2 were conducted over central China in spring 2008, where intense measurements are lacking. A substantial amount of SO2 was observed in the free troposphere, which is important to regional transport and remote sensing. I successfully validated the SO2 columns with satellite retrievals, and proved that the new OMI SO2 algorithm performs better than the conventional algorithm. An emission inventory was evaluated through a combination of model simulations and satellite products. Between 2006 and 2008, the SO2 emissions had been reduced substantially over middle and eastern China. I also analyzed the model simulations, and find the SO2 lifetime is ~ 38 h during spring in China and that ~50% of Chinese emissions are exported to the western Pacific.
AIR POLLUTION EMISSIONS FROM HIGHWAY VEHICLES: QUANTIFYING IMPACTS OF HUMIDITY, AMBIENT TEMPERATURE, AND COVID-19–RELATED TRAVEL RESTRICTIONS
(2022) Hall-Quinlan, Dolly; Dickerson, Russell R; Atmospheric and Oceanic Sciences; Digital Repository at the University of Maryland; University of Maryland (College Park, Md.)
Air pollution adversely affects human health and climate at both local and regional scales. With vehicles representing the dominant source of several important air pollutants, more work is needed to improve our understanding of the factors impacting vehicular emissions to further reduce pollution levels. In this dissertation, I use ambient, near-road (NR) observations of nitrogen oxides (NOx), carbon monoxide (CO), black carbon (BC), carbon dioxide (CO2), and traffic to characterize vehicular emissions and the influence of weather and traffic patterns. The first part focuses on how vehicular emissions respond to ambient temperature. The second part investigates traffic pattern changes resulting from COVID-19 travel restrictions and the effects on mobile emissions.Chapter 2 discusses the temperature and specific humidity sensitivity of vehicular NOx, CO, and CO2 emissions. Using NR (along Interstate 95) observations during the cold season, I calculated hourly ΔCO/ΔNOx, ΔCO2/ΔNOx, and ΔCO2/ΔCO ratios to infer emissions ratios from vehicular exhaust. Chapter 3 builds on this work by extending the temperature analysis to BC emissions using ∆BC/∆CO and ∆BC/∆CO2. Results show a factor of two decrease in NOx (−5°C to 25°C) and a ~50% increase in BC emissions (−5°C to 20°C). Combined with traffic observations, we trace this effect to diesel-powered trucks. The observed trends are then used to evaluate the temperature sensitivity in modeled mobile emissions. Important public policy decisions regarding air quality often depend on models that generate accurate emissions estimates from various sectors, including mobile sources. The US EPA estimates vehicular emissions for air quality models using the MOtor Vehicle Emissions Simulator (MOVES). Our analysis shows that MOVES underestimates the temperature effect in NOx emissions and does not adjust BC emissions, indicating that more work is needed to improve the temperature sensitivity in the model. Chapter 4 examines the impact of changing traffic patterns on I-95 in April 2020 on mobile emissions revealing ~60% fewer on-road cars and ~10% fewer trucks, resulting in faster highway speeds and less stop-and-go traffic. Coupled with an analysis of emission ratios, the results of this study suggest a significant decrease in BC emissions from diesel-powered trucks attributable to improved traffic flow.
Air Pollution Response to Changing Weather and Power Plant Emissions in the Eastern United States
(2008-11-20) Bloomer, Bryan Jaye; Dickerson, Russell R; Atmospheric and Oceanic Sciences; Digital Repository at the University of Maryland; University of Maryland (College Park, Md.)
Air pollution in the eastern United States causes human sickness and death as well as damage to crops and materials. NOX emission reduction is observed to improve air quality. Effectively reducing pollution in the future requires understanding the connections between smog, precursor emissions, weather, and climate change. Numerical models predict global warming will exacerbate smog over the next 50 years. My analysis of 21 years of CASTNET observations quantifies a climate change penalty. I calculate, for data collected prior to 2002, a climate penalty factor of ~3.3 ppb O3/°C across the power plant dominated receptor regions in the rural, eastern U.S. Recent reductions in NOX emissions decreased the climate penalty factor to ~2.2 ppb O3/°C. Prior to 1995, power plant emissions of CO2, SO2, and NOX were estimated with fuel sampling and analysis methods. Currently, emissions are measured with continuous monitoring equipment (CEMS) installed directly in stacks. My comparison of the two methods show CO2 and SO2 emissions are ~5% lower when inferred from fuel sampling; greater differences are found for NOX emissions. CEMS are the method of choice for emission inventories and commodity trading and should be the standard against which other methods are evaluated for global greenhouse gas trading policies. I used CEMS data and applied chemistry transport modeling to evaluate improvements in air quality observed by aircraft during the North American electrical blackout of 2003. An air quality model produced substantial reductions in O3, but not as much as observed. The study highlights weaknesses in the model as commonly used for evaluating a single day event and suggests areas for further investigation. A new analysis and visualization method quantifies local-daily to hemispheric-seasonal scale relationships between weather and air pollution, confirming improved air quality despite increasing temperatures across the eastern U.S. Climate penalty factors indicate amplified smog formation in areas of the world with rising temperatures and increasing emissions. Tools developed in this dissertation provide data for model evaluation and methods for establishing air quality standards with an adequate margin of safety for cleaning the air and protecting the public's health in a world with changing climate.
Aircraft Observations of Dust and Pollutants over NE China: Insight into the Meteorological Mechanisms of Long-Range Transport
(2006) Dickerson, Russell; Li, Can; Li, Zhanqing; Marufu, Lackson; Stehr, Jeffrey; Chen, H.; Wang, P; Xia, X.; Ban, X.; Gong, F.; Yaun, J.; Yang, J.
Substantial concentrations of trace gases and aerosols are lofted and carried from Asia over the Pacific producing an inter-hemispheric impact on atmospheric chemistry and climate. The meteorological mechanism leading to this large-scale transport of dust and pollutants remains a major uncertainty in quantifying the global effects of emissions from the developing world. Models and downwind measurements have identified isentropic advection associated with wave cyclones (warm conveyor belt circulation) as an important mechanism. We present data from a case study conducted over Shenyang in NE China as part of EAST-AIRE in April 2005 in which upstream convection, rather than WCB lofting appears to dominate. Observations from instrumented aircraft flights, back trajectories, and satellite images of clouds (GOES) and aerosols (MODIS) are analyzed. In this heavily industrialized and populated region, the warm-sector PBL air ahead of a cold front was highly polluted. In the free troposphere, between ~1000 and 4000 m altitude, concentrations of trace gases and aerosols were lower, but well above background; we measured ~70 ppb O3, ~300 ppb CO, ~2 ppb SO2, and ~ 8x10-5 m-1 aerosol scattering. These observations show that dry (non-precipitating) convection can be an important mechanism for converting local air pollution problems into regional or global atmospheric chemistry problems. Climatological data indicate that spring (MAM) precipitation over NE China is low, about 90 mm compared to 290 mm over the NE US. Cloud cover, however, is similar with cumulus clouds reported about 7% of the time over NE China and about 9% of the time over the NE US suggesting that lofting in dry convective events may be common over NE Asia. Evaluation of models’ convective schemes and further observations near the source regions are called for.
Analyses of multiple global and regional aerosol products: investigation of aerosol effects and artifacts
(2005-12-02) Jeong, Myeong Jae; Li, Zhanqing; Meteorology; Digital Repository at the University of Maryland; University of Maryland (College Park, Md.)
Multiple aerosol products derived from satellite, ground-based, and air-borne instruments were analyzed with a focus on satellite-based aerosol products. Aerosol measurements based on different techniques were utilized to investigate the effects and the artifacts of aerosols and clouds by taking advantages of respective techniques. The global aerosol products derived from Advanced Very High Resolution Radiometer (AVHRR) and Total Ozone Mapping Spectrometer (TOMS), were analyzed for extracting synergic information. Global distributions of dominant aerosol type(s) were derived and the two products were combined to acquire an extended spatial coverage of aerosol optical thickness (AOT) at a common wavelength (0.55um). It was shown that the derived AOT agreed reasonably with AOT from the state-of-the-art Moderate Resolution Imaging Spectroradiometer (MODIS). In-depth comparison of aerosol products derived from the MODIS and the AVHRR was performed. New insights and understanding were gained for the discrepancies between the two prominent aerosol products, allowing for bridging the current and past products. Several factors causing the discrepancies were investigated. Cloud-screening techniques and aerosol models employed by the retrieval algorithms were found to be the most important factors explaining the observed discrepancies. The column aerosol humidification effect (AHE) was investigated. The column AHE was shown to be sensitive to changes in relative humidity (RH). Six methods to infer the column AHE were introduced. The knowledge of the AHE helps investigate aerosol properties and retrievals near clouds, enabling separation of aerosol real effects from artifacts associated with clouds. Finally, apparent correlations between AOT and cloud amount from ground- and satellite-based measurements were investigated. Several factors including air convergence, cloud contamination and uncertainty in cloud cover estimation, the AHE, cloud-processed/new particle genesis were studied to explain the correlations. We showed that the correlation found in ground-based measurements is mostly due to real effects while satellite-based measurements are significantly influenced by artifacts caused by clouds.
An analysis of convective transport, Lightning NO.sub.x production, and chemistry in midlatitude and subtropical thunderstorms
(2006-10-18) Ott, Lesley Elaine; Dickerson, Russell R.; Atmospheric and Oceanic Sciences; Digital Repository at the University of Maryland; University of Maryland (College Park, Md.)
The impact of lightning NO.sub.x production and convective transport on tropospheric chemistry was studied in four thunderstorms observed during field projects using a 3-dimensional (3-D) cloud-scale chemical transport model (CSCTM). The dynamical evolution of each storm was simulated using a cloud-resolving model, and the output used to drive the off-line CSCTM which includes a parameterized source of lightning NO.sub.x based on observed cloud-to-ground (CG) and intracloud (IC) flash rates. Simulated mixing ratios of tracer species were compared to anvil aircraft observations to evaluate convective transport in the model. The production of NO per CG flash (P.sub.CG) was estimated based on mean observed peak current, and production per IC flash (P.sub.IC) was scaled to P.sub.CG. Different values of P.sub.IC/P.sub.CG were assumed and the results compared with in-cloud aircraft measurements to estimate the ratio most appropriate for each storm. The impact of lightning NO.sub.x on ozone and other species was examined during the storm in the CSCTM and following each storm in the convective plume using a chemistry-only version of the model which includes diffusion but without advection, and assumes clear-sky photolysis rates. New lightning parameterizations were implemented in the CSCTM. One parameterization uses flash length data, rather than flash rates, as input, and production per meter of flash channel length is estimated. A second parameterization simulates indivdual lightning flashes rather than distributing lightning NO_x uniformly among a large number of gridcells to better reproduce the variability of observations. The results suggest that P_IC is likely on the order of P_CG and not significantly less as has been assumed in many global modeling studies. Mean values of P_CG=500 moles NO and P_IC=425 moles NO have been estimated from these simulations of midlatitude and subtropical continental thunderstorms. Based on the estimates of production per flash, and an assumed ratio of the number of IC to CG flashes and global flash rate, a global annual lightning NO source of 8.6 Tg N yr^-1 is estimated. Based on these simulations, vertical profiles of lightning NO_x mass for subtropical and midlatitude continental regimes have been computed for use in global and regional chemical transport models.
Analysis of Summertime PM2.5 and haze in the Mid-Atlantic Region
(Air & Waste Management Association (A&WMA), 2003) Chen, L.-W. Antony; Chow, Judith C.; Doddridge, Bruce G.; Dickerson, Russell R.; Ryan, William F.; Mueller, Peter K.
Observations of the mass and chemical composition of particles less than 2.5 µm in aerodynamic diameter (PM2.5), light extinction, and meteorology in the urban Baltimore-Washington corridor during July 1999 and July 2000 are presented and analyzed to study summertime haze formation in the mid-Atlantic region. The mass fraction of ammoniated sulfate (SO4^2-) and carbonaceous material in PM2.5 were each ~50% for cleaner air (PM2.5 < 10 µg/m3) but changed to ~60% and ~20%, respectively, for more polluted air (PM2.5 > 30 µg/m3). This signifies the role of SO4^2- in haze formation. Comparisons of data from this study with the Interagency Monitoring of Protected Visual Environments network suggest that SO4^2- is more regional than carbonaceous material and originates in part from upwind source regions. The light extinction coefficient is well correlated to PM2.5 mass plus water associated with inorganic salt, leading to a mass extinction efficiency of 7.6 ± 1.7 m2/g for hydrated aerosol. The most serious haze episode occurring between July 15 and 19, 1999, was characterized by westerly transport and recirculation slowing removal of pollutants. At the peak of this episode, 1-hr PM2.5 concentration reached ~45 µg/m3, visual range dropped to ~5 km, and aerosol water likely contributed to ~40% of the light extinction coefficient.
APPLICATION OF NEURAL NETWORKS TO EMULATION OF RADIATION PARAMETERIZATIONS IN GENERAL CIRCULATION MODELS
(2012) Belochitski, Alexei; Baer, Ferdinand; Atmospheric and Oceanic Sciences; Digital Repository at the University of Maryland; University of Maryland (College Park, Md.)
A novel approach based on using neural network (NN) techniques for approximation of physical components of complex environmental systems has been applied and further developed in this dissertation. A new type of a numerical model, a complex hybrid environmental model, based on a combination of deterministic and statistical learning model components, has been explored. Conceptual and practical aspects of developing hybrid models have been formalized as a methodology for applications to climate modeling and numerical weather prediction. The approach uses NN as a machine or statistical learning technique to develop highly accurate and fast emulations for model physics components/parameterizations. The NN emulations of the most time consuming model physics components, short and long wave radiation (LWR and SWR) parameterizations have been combined with the remaining deterministic components of a general circulation model (GCM) to constitute a hybrid GCM (HGCM). The parallel GCM and HGCM simulations produce very similar results but HGCM is significantly faster. The high accuracy, which is of a paramount importance for the approach, and a speed-up of model calculations when using NN emulations, open the opportunity for model improvement. It includes using extended NN ensembles and/or more frequent calculations of full model radiation resulting in an improvement of radiation-cloud interaction, a better consistency with model dynamics and other model physics components. First, the approach was successfully applied to a moderate resolution (T42L26) uncoupled NCAR Community Atmospheric Model driven by climatological SST for a decadal climate simulation mode. Then it has been further developed and subsequently implemented into a coupled GCM, the NCEP Climate Forecast System with significantly higher resolution (T126L64) and time dependent CO2 and tested for decadal climate simulations, seasonal prediction, and short- to medium term forecasts. The developed highly accurate NN emulations of radiation parameterizations are on average one to two orders of magnitude faster than the original radiation parameterizations. The NN approach was extended by introduction of NN ensembles and a compound parameterization with quality control of larger errors. Applicability of other statistical learning techniques, such as approximate nearest neighbor approximation and random trees, to emulation of model physics has also been explored
APPLICATIONS OF ENSEMBLE FORECAST SENSITIVITY TO OBSERVATIONS FOR IMPROVING NUMERICAL WEATHER PREDICTION
(2018) Chen, Tse-Chun; Kalnay, Eugenia; Atmospheric and Oceanic Sciences; Digital Repository at the University of Maryland; University of Maryland (College Park, Md.)
Massive amounts of observations are assimilated every day into modern Numerical Weather Prediction (NWP) systems, and more are being deployed. The large volume of data prevents thorough monitoring and screening (QC) the impact of each assimilated observation using standard observing system experiments (OSEs). The presence of so many observations also makes very difficult to estimate the impact of a new observing system using OSEs. Forecast Sensitivity to Observation using adjoint formulation (AFSO, Langland and Baker, 2004) provides an efficient impact evaluation of each observation on forecasts. We propose 3 applications using the simpler ensemble formulation of FSO (EFSO, Kalnay et al., 2012) to improve NWP, namely (1) online monitoring tool, (2) data selection, and (3) proactive quality control (PQC). We first demonstrate PQC on a simple Lorenz (1996) model, showing that EFSO is able to identify artificially '`flawed" observations. We then show that PQC improves the quality of analysis and forecast of the system, even if the observations are flawless, and the improvement is robust against common sub-optimal of DA configurations in operation. A PQC update method reusing the original Kalman gain is found to be both accurate and computationally efficient. EFSO and PQC are then explored with realistic GFS systems. A close-to-operation GFS-GSI Hybrid En-Var system is used to examine the data monitoring and selection applications. The benefit of the online observation monitoring and data rejection based on EFSO is very apparent. Identifying and deleting detrimental radiance channels results in a forecast improvement. Results obtained on a lower resolution GFS system show that PQC significantly improves the quality of analysis and 5-day forecasts for all variables over the globe. Most of the improvement comes from "cycling" PQC, which accumulates improvements brought by deleting detrimental observations over many cycles, rather than from deleting detrimental observations in the current cycle. Thus we avoid using "future data" in PQC and its implementation is shown to be computationally feasible in NCEP operations.
Applications of the LETKF to adaptive observations, analysis sensitivity, observation impact and the assimilation of moisture
(2007-11-26) Liu, Junjie; Kalnay, Eugenia; Atmospheric and Oceanic Sciences; Digital Repository at the University of Maryland; University of Maryland (College Park, Md.)
In this thesis we explore four new applications of the Local Ensemble Transform Kalman Filter (LETKF), namely adaptive observations, analysis sensitivity, observation impact, and multivariate humidity assimilation. In each of these applications we have obtained promising results. In the adaptive observation studies, we found that ensemble spread strategy, where adaptive observations are selected among the points with largest ensemble spread (with the constraint that observations cannot be contiguous in order to avoid clusters of adaptive observations) is very effective and close to optimal sampling. The application on simulated Doppler Wind Lidar (DWL) adaptive observation studies shows that 3D-Var is as effective as LETKF with 10% adaptive observations sampled with the ensemble spread strategy. With 2% adaptive observations, 3D-Var is not as effective as the LETKF. In the analysis sensitivity study, we proposed to calculate this quantity within the LETKF with low additional computational time. Unlike in 4D-Var (Cardinali et al., 2004), in the LETKF, the computation is exact and satisfies the theoretical value limits (between 0 and 1). The results from simulated experiments show that the trace of analysis sensitivity qualitatively reflects the observation impact obtained from independently computed data addition or data denial OSSE experiments. In the observation impact study, we derived a formula to estimate the impact of observations on short-range forecasts as in Langland and Baker (2004), but without using an adjoint model. Both methods estimate more than 90% accuracy the actual observation impact on the short-range forecast error improvement. Like the adjoint method, the method we proposed detects observations that have either large random error or unaccounted bias. This method can be easily calculated within the LETKF, and provides a powerful tool to estimate the quality of observations. Finally, for the first time, we assimilate humidity observations multivariately in both perfect model experiments and real data assimilation. We found that multivariate assimilation is better than univariate assimilation. The assimilation of pseudo-RH (Dee and da Silva, 2003) is better than the choice of specific humidity and relative humidity. The multivariate assimilation of AIRS specific humidity retrievals on NCEP GFS system shows positive impact on the winds analysis.
APPLICATIONS OF THE OZONE MONITORING INSTRUMENT IN OBSERVING VOLCANIC SULFUR DIOXIDE PLUMES AND SULFATE DEPOSITION
(2021) Fedkin, Niko Markovich; Dickerson, Russell R; Atmospheric and Oceanic Sciences; Digital Repository at the University of Maryland; University of Maryland (College Park, Md.)
Sulfur dioxide (SO2), a gas emitted by both volcanoes and anthropogenic activity, is a major pollutant and a precursor to sulfate aerosols. Sulfates can be deposited back to the ground where they have adverse impact on the environment or reside in the stratosphere as aerosols and affect radiative forcing. I investigated two components that stem from SO2: the deposition of sulfate, and the remote sensing of the SO2 layer height, important for aviation safety and chemical modeling. In the first study, I used column SO2 data from the Ozone Monitoring Instrument (OMI), and sulfate wet deposition data from the National Atmospheric Deposition Program to investigate the temporal and spatial relationship between trends in SO2 emissions and the downward sulfate wet deposition over the northeastern U.S. from 2005 to 2015. The results showed that emission reductions are reflected in deposition reductions within this same region. Emission reductions along the Ohio River Valley led to decreases in sulfate deposition not only in eastern OH and western PA, but also further downwind at sites in Delaware and Maryland. The findings suggested that emissions and wet deposition are linked through not only the location of sources relative to the observing sites, but also photochemistry and weather patterns characteristic to the region in winter and summer. The second part of this dissertation focuses on SO2 layer height retrievals and their applications. To this end I applied the Full Physics Inverse Learning Machine (FP-ILM) algorithm to OMI radiances in the spectral range of 310-330 nm. This approach utilized radiative transfer calculations to generate a large dataset of synthetic radiance spectra for a wide range of geophysical parameters. The spectral information was then used to train a neural network to predict the SO2 height. The main advantage of the algorithm is its speed, retrieving plume height in less than 10 min for an entire OMI orbit. I also compared the SO2 height retrievals to other data sources and explored some potential applications, in particular their use in volcanic SO2 plume forecasts and estimating the total mass emitted from volcanic eruptions.
Assessing Coastal SMAP Surface Salinity Accuracy and Its Application to Monitoring Gulf of Maine Circulation Dynamics
(MDPI, 2018-08-06) Grodsky, Semyon A.; Vandemark, Douglas; Feng, Hui
Monitoring the cold and productive waters of the Gulf of Maine and their interactions with the nearby northwestern (NW) Atlantic shelf is important but challenging. Although remotely sensed sea surface temperature (SST), ocean color, and sea level have become routine, much of the water exchange physics is reflected in salinity fields. The recent invention of satellite salinity sensors, including the Soil Moisture Active Passive (SMAP) radiometer, opens new prospects in regional shelf studies. However, local sea surface salinity (SSS) retrieval is challenging due to both cold SST limiting salinity sensor sensitivity and proximity to land. For the NW Atlantic, our analysis shows that SMAP SSS is subject to an SST-dependent bias that is negative and amplifies in winter and early spring due to the SST-related drop in SMAP sensor sensitivity. On top of that, SMAP SSS is subject to a land contamination bias. The latter bias becomes noticeable and negative when the antenna land contamination factor (LC) exceeds 0.2%, and attains maximum negative values at LC = 0.4%. Coastward of LC = 0.5%, a significant positive land contamination bias in absolute SMAP SSS is evident. SST and land contamination bias components are seasonally dependent due to seasonal changes in SST/winds and terrestrial microwave properties. Fortunately, it is shown that SSS anomalies computed relative to a satellite SSS climatology can effectively remove such seasonal biases along with the real seasonal cycle. SMAP monthly SSS anomalies have sufficient accuracy and applicability to extend nearer to the coasts. They are used to examine the Gulf of Maine water inflow, which displayed important water intrusions in between Georges Banks and Nova Scotia in the winters of 2016/17 and 2017/18. Water intrusion patterns observed by SMAP are generally consistent with independent measurements from the European Soil Moisture Ocean Salinity (SMOS) mission. Circulation dynamics related to the 2016/2017 period and enhanced wind-driven Scotian Shelf transport into the Gulf of Maine are discussed.
The Assimilation of Hyperspectral Satellite Radiances in Global Numerical Weather Prediction
(2008-04-29) Jung, James Alan; Kalnay, Eugenia; Le Marshall, John F.; Atmospheric and Oceanic Sciences; Digital Repository at the University of Maryland; University of Maryland (College Park, Md.)
Hyperspectral infrared radiance data present opportunities for significant improvements in data assimilation and Numerical Weather Prediction (NWP). The increase in spectral resolution available from the Atmospheric Infrared Sounder (AIRS) sensor, for example, will make it possible to improve the accuracy of temperature and moisture fields. Improved accuracy of the NWP analyses and forecasts should result. In this thesis we incorporate these hyperspectral data, using new assimilation methods, into the National Centers for Environmental Prediction's (NCEP) operational Global Data Assimilation System/Global Forecast System (GDAS/GFS) and investigate their impact on the weather analysis and forecasts. The spatial and spectral resolution of AIRS data used by NWP centers was initially based on theoretical calculations. Synthetic data were used to determine channel selection and spatial density for real time data assimilation. Several problems were previously not fully addressed. These areas include: cloud contamination, surface related issues, dust, and temperature inversions. In this study, several improvements were made to the methods used for assimilation. Spatial resolution was increased to examine every field of view, instead of one in nine or eighteen fields of view. Improved selection criteria were developed to find the best profile for assimilation from a larger sample. New cloud and inversion tests were used to help identify the best profiles to be assimilated in the analysis. The spectral resolution was also increased from 152 to 251 channels. The channels added were mainly near the surface, in the water vapor absorption band, and in the shortwave region. The GFS was run at or near operational resolution and contained all observations available to the operational system. For each experiment the operational version of the GFS was used during that time. The use of full spatial and enhanced spectral resolution data resulted in the first demonstration of significant impact of the AIRS data in both the Northern and Southern Hemisphere. Experiments were performed to show the contribution to the improvements in global weather forecasts from the increase in spatial and spectral resolution. Both spatial and spectral resolution increases were shown to make significant contributions to forecast skill. New methods were also developed to check for clouds, inversions and for estimating surface emissivity. Overall, an improved methodology for assimilating hyperspectral AIRS data was achieved.