Atmospheric & Oceanic Science Research Works

Permanent URI for this collectionhttp://hdl.handle.net/1903/1596

Formerly known as the Department of Meteorology.

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OMI Satellite LNOx* VCD June 11, 2012
(2024) Seiler, Madilynn; Buscela, Eric; Pickering, Kenneth
1ºx1º gridded OMI Vertical Column Densities of Lightning NOx without background subtraction for June 11th, 2012
Climate change quadruples flood-causing extreme monsoon rainfall events in Bangladesh and northeast India
(Wiley, 2023-12-22) Fahad, Abdullah A.; Hasan, Mahdi; Sharmili, Noshin; Islam, Shammunul; Swenson, Erik T.; Roxy, M. K.
Bangladesh and northeast India are the most densely populated regions in the world where severe floods as a result of extreme rainfall events kill hundreds of people and cause socio-economic losses regularly. Owing to local high topography, the moisture-carrying monsoon winds converge near southeast Bangladesh (SEB) and northeast Bangladesh and India (NEBI), which produces significant extreme rainfall events from May to October. Using observed data, we find an increasing trend of 1-day extreme event (>150 mm/day-1) frequency during 1950–2021. The extreme rainfall events quadrupled over western Meghalaya (affecting NEBI) and coastal SEB during this period. Composite analysis indicates that warm Bay of Bengal sea-surface temperature intensifies the lower tropospheric moisture transport and flux through the low-level jet (LLJ) to inland, where mountain-forced moisture converges and precipitates as rainfall during extreme events. To understand the role of climate change, we use high-resolution downscaled models from Coupled Model Intercomparison Project phase 6 (CMIP6). We find that the monsoon extreme event increase is ongoing and the region of quadrupled events further extends over the NEBI and SEB in the future (2050–2079) compared with historical simulations (1950–1979). A quadrupling of the intense daily moisture transport episodes due to increased LLJ instability, a northward shift of LLJ, and increased moisture contribute to the increased future extreme events. This dynamic process causes moisture to be transported to the NEBI from the southern Bay of Bengal, and the local thermodynamic response to climate change contributes to the increased extreme rainfall events. The CMIP6 projection indicates that more devastating flood-causing extreme rainfall events will become more frequent in the future.
Understanding the Effects of Aerosols on Electrification and Lightning Polarity in an Idealized Supercell Thunderstorm via Model Emulation
(Wiley, 2023-12-29) Sun, Mengyu; Li, Zhanqing; Wang, Tao; Mansell, Edward R.; Qie, Xiushu; Shan, Siyu; Liu, Dongxia; Cribb, Maureen
Aerosol effects on the lightning intensity and polarity of a continental supercell storm were investigated using a three-dimensional lightning scheme within the Weather Research and Forecasting model. We find that both intra-cloud (IC) and cloud-to-ground (CG) flashes are enhanced by the increasing number of cloud condensation nuclei (CCN), especially the percentage of positive CG (+CG) strokes peaking at 42%. Electrical characteristics of the storm varied in different aerosol scenarios through microphysical processes. Added aerosols increase the number of cloud droplets and ice-phase hydrometeors. The greater ice-crystal concentration and larger graupel size ensure sufficient charge separation, leading to higher charge density and more lightning discharges. In addition, an inverted polarity charge structure with a strong positive-charge region in the mid-levels was formed mainly due to the positively charged graupel in the presence of higher supercooled cloud water content. Positive lightning channels originating from this positive-charge region propagated to the ground, producing more +CG strokes. When the aerosol concentration was low, the charge density in the upper positive-charge region was much lower due to smaller ice-particle content. Consequently, there were barely any +CG strokes. Most of the negative CG flashes deposited positive charge in the lower negative-charge region.
On the Role of Indian Ocean SST in Influencing the Differences in Atmospheric Variability Between 2020–2021 and 2021–2022 La Niña Boreal Winters
(Wiley, 2024-03-10) Zhang, Tao; Kumar, Arun
The difference in observed atmospheric anomalies over the Northern Hemisphere winter between 2021–22 and 2020–21 La Niña years indicated a tripole pattern consisting of a Japan cyclone, a Bering Sea anticyclone, and a cyclone over the North American continent. This feature, however, was not replicated in the North American Multi-Model Ensemble (NMME) forecasts. A set of model sensitivity experiments was performed to better understand the cause of this discrepancy. The results revealed the possible role of the influence of sea surface temperature (SST) anomalies, particularly over the Indian Ocean, on the observed circulation differences that was further modulated by internal atmospheric variability. The failure in predicting circulation changes in NMME was next attributed to the errors in SST predictions over the Indian Ocean and highlights the need for improvements in SST forecasts over this region.
Evaluation of Stratocumulus Evolution Under Contrasting Temperature Advections in CESM2 Through a Lagrangian Framework
(Wiley, 2024-02-16) Zhang, Haipeng; Zheng, Youtong; Li, Zhanqing
This study leveraged a Lagrangian framework to examine the evolution of stratocumulus clouds under cold and warm advections (CADV and WADV) in the Community Earth System Model 2 (CESM2) against observations. We found that CESM2 simulates a too rapid decline in low-cloud fraction (LCF) and cloud liquid water path (CLWP) under CADV conditions, while it better aligns closely with observed LCF under WADV conditions but overestimates the increase in CLWP. Employing an explainable machine learning approach, we found that too rapid decreases in LCF and CLWP under CADV conditions are related to overestimated drying effects induced by sea surface temperature, whereas the substantial increase in CLWP under WADV conditions is associated with the overestimated moistening effects due to free-tropospheric moisture and surface winds. Our findings suggest that overestimated drying effects of sea surface temperature on cloud properties might be one of crucial causes for the high equilibrium climate sensitivity in CESM2.
On the use of consistent bias corrections to enhance the impact of Aeolus Level-2B Rayleigh winds on National Oceanic and Atmospheric Administration global forecast skill
(Wiley, 2023-10-14) Liu, Hui; Garrett, Kevin; Ide, Kayo; Hoffman, Ross N.
The operational Aeolus Level-2B (L2B) horizontal line-of-sight (HLOS) retrieved Rayleigh winds, produced by the European Space Agency (ESA), utilize European Centre for Medium-Range Weather Forecasts (ECMWF) short-term forecasts of temperature, pressure, and horizontal winds in the Rayleigh–Brillouin and M1 correction procedures. These model fields or backgrounds can contain ECMWF model-specific errors, which may propagate to the retrieved Rayleigh winds. This study examines the sensitivity of the retrieved Rayleigh winds to the changes in the model backgrounds, and the potential benefit of using the same system, in this case the National Oceanic and Atmospheric Administration's Finite-Volume Cubed Sphere Global Forecast System (FV3GFS), for both the corrections and the data assimilation and forecast procedures. It is shown that the differences in the model backgrounds (FV3GFS minus ECMWF) can propagate through the Level-2B horizontal line-of-sight Rayleigh wind retrieval process, mainly the M1 correction, resulting in differences in the retrieved Rayleigh winds with mean and standard deviation of magnitude as large as 0.2 m·s−1. The differences reach up to 0.4, 0.6, and 0.7 m·s−1 for the 95th, 99th, and 99.5th percentiles of the sample distribution with maxima of ∼1.4 m·s−1. The numbers of the large differences for the combined lower and upper 5th, 1st, and 0.5th percentile pairs are ∼6,100, 1,220, and 610 between 2.5 and 25 km height globally per day respectively. The ESA-disseminated Rayleigh wind product (based on the ECMWF corrections) already shows a significant positive impact on the FV3GFS global forecasts. In the observing system experiments performed, compared with the ESA Rayleigh winds, the use of the FV3GFS-corrected Rayleigh winds lead to ∼0.5% more Rayleigh winds assimilated in the lower troposphere and show enhanced positive impact on FV3GFS forecasts at the day 1–10 range but limited to the Southern Hemisphere.
Flood Impacts on Net Ecosystem Exchange in the Midwestern and Southern United States in 2019
(Wiley, 2023-09-06) Balashov, Nikolay V.; Ott, Lesley E.; Weir, Brad; Basu, Sourish; Davis, Kenneth J.; Miles, Natasha L.; Thompson, Anne M.; Stauffer, Ryan M.
Climate extremes such as droughts, floods, heatwaves, frosts, and windstorms add considerable variability to the global year-to-year increase in atmospheric CO2 through their influence on terrestrial ecosystems. While the impact of droughts on terrestrial ecosystems has received considerable attention, the response to flooding is not well understood. To improve upon this knowledge, the impact of the 2019 anomalously wet conditions over the Midwest and Southern US on CO2 vegetation fluxes is examined in the context of 2017–2018 when such precipitation anomalies were not observed. CO2 is simulated with NASA's Global Earth Observing System (GEOS) combined with the Low-order Flux Inversion, where fluxes of CO2 are estimated using a suite of remote sensing measurements including greenness, night lights, and fire radiative power as well as with a bias correction based on insitu observations. Net ecosystem exchange CO2 tracers are separated into the three regions covering the Midwest, South, and Eastern Texas and adjusted to match CO2 observations from towers located in Iowa, Mississippi, and Texas. Results indicate that for the Midwestern region consisting primarily of corn and soybeans crops, flooding contributes to a 15%–25% reduction of annual net carbon uptake in 2019 in comparison to 2017 and 2018. These results are supported by independent reports of changes in agricultural activity. For the Southern region, comprised mainly of non-crop vegetation, annual net carbon uptake is enhanced in 2019 by about 10%–20% in comparison to 2017 and 2018. These outcomes show the heterogeneity in effects that excess wetness can bring to diverse ecosystems.
Systematic Validation of Ensemble Cloud-Process Simulations Using Polarimetric Radar Observations and Simulator Over the NASA Wallops Flight Facility
(Wiley, 2023-08-18) Matsui, Toshi; Wolff, David B.; Lang, Stephen; Mohr, Karen; Zhang, Minghua; Xie, Shaocheng; Tang, Shuaiqi; Saleeby, Stephen M.; Posselt, Derek J.; Braun, Scott A.; Chern, Jiun-Dar; Dolan, Brenda; Pippitt, Jason L.; Loftus, Adrian M.
The BiLateral Operational Storm-Scale Observation and Modeling (BLOSSOM) project was initiated to establish a long-term supersite to improve understanding of cloud physical states and processes as well as to support satellite and climate model programs over the Wallops Flight Facility site via a bilateral approach of storm-scale observations and process modeling. This study highlights a noble systematic validation framework of the BLOSSOM ensemble cloud-process simulations through mixed-phase, light-rain, and deep-convective precipitation cases. The framework consists of creating a domain-shifted ensemble of large-scale forcing data sets, and configuring and performing cloud-process simulations with three different bulk microphysics schemes. Validation uses NASA S-band dual-POLarimetric radar observations in the form of statistical composites and skill scores via a polarimetric radar simulator and newly developed CfRad Data tool (CfRAD). While the simulations capture the overall structures of the reflectivity composites, polarimetric signals are still poorly simulated, mainly due to a lack of representation of ice microphysics diversity in shapes, orientation distributions, and their complex mixtures. Despite the limitation, this new ensemble-based validation framework demonstrates that (a) no particular forcing or microphysics scheme outperforms the rest and (b) the skill scores of coarse- and fine-resolution ensemble simulations with different domain-shifted forcing and microphysics schemes are highly correlated with each other with no clear improvement. On the other hand, this suggests that coarse-resolution ensemble simulations are relevant for selecting the best meteorological forcing and microphysics scheme before conducting computationally demanding large eddy simulations in support of aircraft and satellite instrument development as well as cloud-precipitation-convection parameterizations.
A Study of the Oklahoma City Urban Heat Island Effect Using a WRF/Single-Layer Urban Canopy Model, a Joint Urban 2003 Field Campaign, and MODIS Satellite Observations
(MDPI, 2017-09-07) Zhang, Hengyue; Jin, Menglin S.; Leach, Martin
The urban heat island effect (UHI) for inner land regions was investigated using satellite data, ground observations, and simulations with an Single-Layer Urban Canopy Parameterization (SLUCP) coupled into the regional Weather Research Forecasting model (WRF, http://wrf-model.org/index.php). Specifically, using the satellite-observed surface skin temperatures (Tskin), the intensity of the UHI was first compared for two inland cities (Xi’an City, China, and Oklahoma City (OKC)), which have different city populations and building densities. The larger population density and larger building density in Xi’an lead to a stronger skin-level UHI by 2 °C. However, the ground observed 2 m surface air temperature (Tair) observations showed an urban cooling island effect (UCI) over the downtown region in OKC during the daytime of 19 July 2003, from a DOE field campaign (Joint Urban 2003). To understand this contrast between satellite-based Tskin and ground-based Tair, a sensitivity study using WRF/SLUCP was analyzed. The model reproduced a UCI in OKC. Furthermore, WRF/Noah/SLUCM simulations were also compared with the Joint Urban 2003 ground observations, including wind speeds, wind directions, and energy fluxes. Although the WRF/SLUCM model failed to simulate these variables accurately, it reproduced the diurnal variations of surface temperatures, wind speeds, wind directions, and energy fluxes reasonably well.
Assessing Coastal SMAP Surface Salinity Accuracy and Its Application to Monitoring Gulf of Maine Circulation Dynamics
(MDPI, 2018-08-06) Grodsky, Semyon A.; Vandemark, Douglas; Feng, Hui
Monitoring the cold and productive waters of the Gulf of Maine and their interactions with the nearby northwestern (NW) Atlantic shelf is important but challenging. Although remotely sensed sea surface temperature (SST), ocean color, and sea level have become routine, much of the water exchange physics is reflected in salinity fields. The recent invention of satellite salinity sensors, including the Soil Moisture Active Passive (SMAP) radiometer, opens new prospects in regional shelf studies. However, local sea surface salinity (SSS) retrieval is challenging due to both cold SST limiting salinity sensor sensitivity and proximity to land. For the NW Atlantic, our analysis shows that SMAP SSS is subject to an SST-dependent bias that is negative and amplifies in winter and early spring due to the SST-related drop in SMAP sensor sensitivity. On top of that, SMAP SSS is subject to a land contamination bias. The latter bias becomes noticeable and negative when the antenna land contamination factor (LC) exceeds 0.2%, and attains maximum negative values at LC = 0.4%. Coastward of LC = 0.5%, a significant positive land contamination bias in absolute SMAP SSS is evident. SST and land contamination bias components are seasonally dependent due to seasonal changes in SST/winds and terrestrial microwave properties. Fortunately, it is shown that SSS anomalies computed relative to a satellite SSS climatology can effectively remove such seasonal biases along with the real seasonal cycle. SMAP monthly SSS anomalies have sufficient accuracy and applicability to extend nearer to the coasts. They are used to examine the Gulf of Maine water inflow, which displayed important water intrusions in between Georges Banks and Nova Scotia in the winters of 2016/17 and 2017/18. Water intrusion patterns observed by SMAP are generally consistent with independent measurements from the European Soil Moisture Ocean Salinity (SMOS) mission. Circulation dynamics related to the 2016/2017 period and enhanced wind-driven Scotian Shelf transport into the Gulf of Maine are discussed.
Tidal Mixing Signatures in the Hong Kong Coastal Waters from Satellite-Derived Sea Surface Temperature
(MDPI, 2018-12-20) Susanto, R. Dwi; Pan, Jiayi; Devlin, Adam T.
Tidal mixing in the coastal waters of Hong Kong was investigated using a combination of in situ observations and high-resolution satellite-derived sea surface temperature (SST) data. An indicator of tide-induced mixing is a fortnightly (spring-neap cycle) signature in SST due to nonlinear interactions between the two principal diurnal and the two principal semi-diurnal tides. Both semi-diurnal and diurnal tides have strong tidal amplitudes and currents near Hong Kong. As a result, both the near-fortnightly (Mf) and fortnightly (MSf) tides are enhanced due to nonlinear tidal signal interactions. In addition, these fortnightly tidal signals are modulated by seasonal variability, with the maximum seasonal modulation of fortnightly tides occurring during the monsoon transition periods in May and October. The largest fortnightly signals are found in the southwestern part of the Pearl River estuary. Tidal constituent properties vary by space and depth, and high-resolution SST plays a pivotal role in resolving the spatial characteristics of tidal mixing.
Validation and Improvement of the WRF Building Environment Parametrization (BEP) Urban Scheme
(MDPI, 2019-09-10) Gohil, Kanishk; Jin, Menglin S.
The building environment parameterization scheme (BEP) is a built-in “urban physics” scheme in the weather research and forecasting (WRF) model. The urbanized College Park (CP) in Maryland state (MD) in the United States (US) covers an approximate land area of 14.8 km2 and has a population of 32,000 (reported by The United States Census Bureau, as of 2017). This study was an effort to validate and improve the BEP urban physics scheme for a small urban setting, College Park, MD. Comparing the WRF/BEP-simulated two-meter air temperatures with the local rooftop WeatherBug® observations and with the airport observations, systemic deficiencies in BEP for urban heat island effect simulation are evident. Specifically, WRF/BEP overestimates the two-meter air temperature by about 10 °F during clear summer nights and slightly underestimates it during noon of the same days by about 1–3 °F. Similar deficiencies in skin temperature simulations are also evident in WRF/BEP. Modification by adding an anthropogenic heat flux term resulted in better estimates for both skin and two-meter air temperatures on diurnal and seasonal scales.
Towards a Unified and Coherent Land Surface Temperature Earth System Data Record from Geostationary Satellites
(MDPI, 2019-06-12) Pinker, Rachel T.; Ma, Yingtao; Chen, Wen; Hulley, Glynn; Borbas, Eva; Islam, Tanvir; Hain, Chris; Cawse-Nicholson, Kerry; Hook, Simon; Basara, Jeff
Our objective is to develop a framework for deriving long term, consistent Land Surface Temperatures (LSTs) from Geostationary (GEO) satellites that is able to account for satellite sensor updates. Specifically, we use the Radiative Transfer for TOVS (RTTOV) model driven with Modern-Era Retrospective Analysis for Research and Applications (MERRA-2) information and Combined ASTER and MODIS Emissivity over Land (CAMEL) products. We discuss the results from our comparison of the Geostationary Operational Environmental Satellite East (GOES-E) with the MODIS Land Surface Temperature and Emissivity (MOD11) products, as well as several independent sources of ground observations, for daytime and nighttime independently. Based on a six-year record at instantaneous time scale (2004–2009), most LST estimates are within one std from the mean observed value and the bias is under 1% of the mean. It was also shown that at several ground sites, the diurnal cycle of LST, as averaged over six years, is consistent with a similar record generated from satellite observations. Since the evaluation of the GOES-E LST estimates occurred at every hour, day and night, the data are well suited to address outstanding issues related to the temporal variability of LST, specifically, the diurnal cycle and the amplitude of the diurnal cycle, which are not well represented in LST retrievals form Low Earth Orbit (LEO) satellites.
The College Park, Maryland, Tornado of 24 September 2001
(MDPI, 2019-10-22) Pryor, Kenneth L.; Wawrzyniak, Tyler; Zhang, Da-Lin
The 24 September 2001 College Park, Maryland, tornado was a long-track and strong tornado that passed within a close range of two Doppler radars. It was the third in a series of three tornadoes associated with a supercell storm that developed in Stafford County, Virginia, and initiated 3–4 km southwest of College Park and dissipated near Columbia, Howard County. The supercell tracked approximately 120 km and lasted for about 126 min. This study presents a synoptic and mesoscale overview of favorable conditions and forcing mechanisms that resulted in the severe convective outbreak associated with the College Park tornado. The results show many critical elements of the tornadic event, including a negative-tilted upper-level trough over the Ohio Valley, a jet stream with moderate vertical shear, a low-level warm, moist tongue of the air associated with strong southerly flow over south-central Maryland and Virginia, and significantly increased convective available potential energy (CAPE) during the late afternoon hours. A possible role of the urban heat island effects from Washington, DC, in increasing CAPE for the development of the supercell is discussed. Satellite imagery reveals the banded convective morphology with high cloud tops associated with the supercell that produced the College Park tornado. Operational WSR-88D data exhibit a high reflectivity “debris ball” or tornadic debris signature (TDS) within the hook echo, the evolution of the parent storm from a supercell structure to a bow echo, and a tornado cyclone signature (TCS). Many of the mesoscale features could be captured by contemporary numerical model analyses. This study concludes with a discussion of the effectiveness of the coordinated use of satellite and radar observations in the operational environment of nowcasting severe convection.
Impact of Fire Emissions on U.S. Air Quality from 1997 to 2016–A Modeling Study in the Satellite Era
(MDPI, 2020-03-12) Tao, Zhining; He, Hao; Sun, Chao; Tong, Daniel; Liang, Xin-Zhong
A regional modeling system that integrates the state-of-the-art emissions processing (SMOKE), climate (CWRF), and air quality (CMAQ) models has been combined with satellite measurements of fire activities to assess the impact of fire emissions on the contiguous United States (CONUS) air quality during 1997–2016. The system realistically reproduced the spatiotemporal distributions of the observed meteorology and surface air quality, with a slight overestimate of surface ozone (O3) by ~4% and underestimate of surface PM2.5 by ~10%. The system simulation showed that the fire impacts on primary pollutants such as CO were generally confined to the fire source areas but its effects on secondary pollutants like O3 spread more broadly. The fire contribution to air quality varied greatly during 1997-2016 and occasionally accounted for more than 100 ppbv of monthly mean surface CO and over 20 µg m−3 of monthly mean PM2.5 in the Northwest U.S. and Northern California, two regions susceptible to frequent fires. Fire emissions also had implications on air quality compliance. From 1997 to 2016, fire emissions increased surface 8-hour O3 standard exceedances by 10% and 24-hour PM2.5 exceedances by 33% over CONUS.
Hygroscopicity of Different Types of Aerosol Particles: Case Studies Using Multi-Instrument Data in Megacity Beijing, China
(MDPI, 2020-03-01) Wu, Tong; Li, Zhanqing; Chen, Jun; Wang, Yuying; Wu, Hao; Jin, Xiao'ai; Liang, Chen; Li, Shangze; Wang, Wei; Cribb, Maureen
Water uptake by aerosol particles alters its light-scattering characteristics significantly. However, the hygroscopicities of different aerosol particles are not the same due to their different chemical and physical properties. Such differences are explored by making use of extensive measurements concerning aerosol optical and microphysical properties made during a field experiment from December 2018 to March 2019 in Beijing. The aerosol hygroscopic growth was captured by the aerosol optical characteristics obtained from micropulse lidar, aerosol chemical composition, and aerosol particle size distribution information from ground monitoring, together with conventional meteorological measurements. Aerosol hygroscopicity behaves rather distinctly for mineral dust coarse-mode aerosol (Case I) and non-dust fine-mode aerosol (Case II) in terms of the hygroscopic enhancement factor, 𝑓𝛽(𝑅𝐻,𝜆532), calculated for the same humidity range. The two types of aerosols were identified by applying the polarization lidar photometer networking method (POLIPHON). The hygroscopicity for non-dust aerosol was much higher than that for dust conditions with the 𝑓𝛽(𝑅𝐻,𝜆532) being around 1.4 and 3.1, respectively, at the relative humidity of 86% for the two cases identified in this study. To study the effect of dust particles on the hygroscopicity of the overall atmospheric aerosol, the two types of aerosols were identified and separated by applying the polarization lidar photometer networking method in Case I. The hygroscopic enhancement factor of separated non-dust fine-mode particles in Case I had been significantly strengthened, getting closer to that of the total aerosol in Case II. These results were verified by the hygroscopicity parameter, κ (Case I non-dust particles: 0.357 ± 0.024; Case II total: 0.344 ± 0.026), based on the chemical components obtained by an aerosol chemical speciation instrument, both of which showed strong hygroscopicity. It was found that non-dust fine-mode aerosol contributes more during hygroscopic growth and that non-hygroscopic mineral dust aerosol may reduce the total hygroscopicity per unit volume in Beijing.
Wildfire Smoke Particle Properties and Evolution, from Space-Based Multi-Angle Imaging
(MDPI, 2020-02-26) Noyes, Katherine Junghenn; Kahn, Ralph; Sedlacek, Arthur; Kleinman, Lawrence; Limbacher, James; Li, Zhanqing
Emitted smoke composition is determined by properties of the biomass burning source and ambient ecosystem. However, conditions that mediate the partitioning of black carbon (BC) and brown carbon (BrC) formation, as well as the spatial and temporal factors that drive particle evolution, are not understood adequately for many climate and air-quality related modeling applications. In situ observations provide considerable detail about aerosol microphysical and chemical properties, although sampling is extremely limited. Satellites offer the frequent global coverage that would allow for statistical characterization of emitted and evolved smoke, but generally lack microphysical detail. However, once properly validated, data from the National Aeronautics and Space Administration (NASA) Earth Observing System’s Multi-Angle Imaging Spectroradiometer (MISR) instrument can create at least a partial picture of smoke particle properties and plume evolution. We use in situ data from the Department of Energy’s Biomass Burning Observation Project (BBOP) field campaign to assess the strengths and limitations of smoke particle retrieval results from the MISR Research Aerosol (RA) retrieval algorithm. We then use MISR to characterize wildfire smoke particle properties and to identify the relevant aging factors in several cases, to the extent possible. The RA successfully maps qualitative changes in effective particle size, light absorption, and its spectral dependence, when compared to in situ observations. By observing the entire plume uniformly, the satellite data can be interpreted in terms of smoke plume evolution, including size-selective deposition, new-particle formation, and locations within the plume where BC or BrC dominates.
The Urban–Rural Heterogeneity of Air Pollution in 35 Metropolitan Regions across China
(MDPI, 2020-07-19) Han, Wenchao; Li, Zhanqing; Guo, Jianping; Su, Tianning; Chen, Tianmeng; Wei, Jing; Cribb, Maureen
Urbanization and air pollution are major anthropogenic impacts on Earth’s environment, weather, and climate. Each has been studied extensively, but their interactions have not. Urbanization leads to a dramatic variation in the spatial distribution of air pollution (fine particles) by altering surface properties and boundary-layer micrometeorology, but it remains unclear, especially between the centers and suburbs of metropolitan regions. Here, we investigated the spatial variation, or inhomogeneity, of air quality in urban and rural areas of 35 major metropolitan regions across China using four different long-term observational datasets from both ground-based and space-borne observations during the period 2001–2015. In general, air pollution in summer in urban areas is more serious than in rural areas. However, it is more homogeneously polluted, and also more severely polluted in winter than that in summer. Four factors are found to play roles in the spatial inhomogeneity of air pollution between urban and rural areas and their seasonal differences: (1) the urban–rural difference in emissions in summer is slightly larger than in winter; (2) urban structures have a more obvious association with the spatial distribution of aerosols in summer; (3) the wind speed, topography, and different reductions in the planetary boundary layer height from clean to polluted conditions have different effects on the density of pollutants in different seasons; and (4) relative humidity can play an important role in affecting the spatial inhomogeneity of air pollution despite the large uncertainties.
Wildfire Smoke Particle Properties and Evolution, From Space-Based Multi-Angle Imaging II: The Williams Flats Fire during the FIREX-AQ Campaign
(MDPI, 2020-11-21) Junghenn Noyes, Katherine T.; Kahn, Ralph A.; Limbacher, James A.; Li, Zhanqing; Fenn, Marta A.; Giles, David M.; Hair, Johnathan W.; Katich, Joseph M.; Moore, Richard H.; Robinson, Claire E.; Sanchez, Kevin J.; Shingler, Taylor J.; Thornhill, Kenneth L.; Wiggins, Elizabeth B.; Winstead, Edward L.
Although the characteristics of biomass burning events and the ambient ecosystem determine emitted smoke composition, the conditions that modulate the partitioning of black carbon (BC) and brown carbon (BrC) formation are not well understood, nor are the spatial or temporal frequency of factors driving smoke particle evolution, such as hydration, coagulation, and oxidation, all of which impact smoke radiative forcing. In situ data from surface observation sites and aircraft field campaigns offer deep insight into the optical, chemical, and microphysical traits of biomass burning (BB) smoke aerosols, such as single scattering albedo (SSA) and size distribution, but cannot by themselves provide robust statistical characterization of both emitted and evolved particles. Data from the NASA Earth Observing System’s Multi-Angle Imaging SpectroRadiometer (MISR) instrument can provide at least a partial picture of BB particle properties and their evolution downwind, once properly validated. Here we use in situ data from the joint NOAA/NASA 2019 Fire Influence on Regional to Global Environments Experiment-Air Quality (FIREX-AQ) field campaign to assess the strengths and limitations of MISR-derived constraints on particle size, shape, light-absorption, and its spectral slope, as well as plume height and associated wind vectors. Based on the satellite observations, we also offer inferences about aging mechanisms effecting downwind particle evolution, such as gravitational settling, oxidation, secondary particle formation, and the combination of particle aggregation and condensational growth. This work builds upon our previous study, adding confidence to our interpretation of the remote-sensing data based on an expanded suite of in situ measurements for validation. The satellite and in situ measurements offer similar characterizations of particle property evolution as a function of smoke age for the 06 August Williams Flats Fire, and most of the key differences in particle size and absorption can be attributed to differences in sampling and changes in the plume geometry between sampling times. Whereas the aircraft data provide validation for the MISR retrievals, the satellite data offer a spatially continuous mapping of particle properties over the plume, which helps identify trends in particle property downwind evolution that are ambiguous in the sparsely sampled aircraft transects. The MISR data record is more than two decades long, offering future opportunities to study regional wildfire plume behavior statistically, where aircraft data are limited or entirely lacking.
Diurnal Variability of Surface Temperature over Lakes: Case Study for Lake Huron
(MDPI, 2021-02-13) Chen, Wen; Pinker, Rachel T.; Rivera, Gerardo; Hook, Simon
The significance of the diurnal variability of Lake Surface Temperature (LST) has been recognized; yet, its magnitude in terms of spatial and temporal variability is not well known. Attempts have been made to derive such information from satellites at a high spatial resolution; however, most have been made from polar orbiting satellites that sample only twice per day. We have developed an approach to derive such information from geostationary satellites at an hourly time scale and at a spatial resolution of about 5 km. The approach to derive LST uses the Radiative Transfer for TIROS Operational Vertical Sounder (TOVS) (RTTOV) model driven by the Modern-Era Retrospective analysis for Research and Applications (MERRA)-2 information. The methodology has been implemented over Lake Huron for about six years. We present the results of the evaluation against various independent satellite products and demonstrate that there is a strong diurnal variability in the skin temperature over the lake and that the lowest and highest values, as derived twice per day from polar orbiting satellites, may not represent the magnitude of the Diurnal Temperature Range (DTR).

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