Atmospheric & Oceanic Science

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Formerly known as the Department of Meteorology.

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    Wildfire Smoke Particle Properties and Evolution, from Space-Based Multi-Angle Imaging
    (MDPI, 2020-02-26) Noyes, Katherine Junghenn; Kahn, Ralph; Sedlacek, Arthur; Kleinman, Lawrence; Limbacher, James; Li, Zhanqing
    Emitted smoke composition is determined by properties of the biomass burning source and ambient ecosystem. However, conditions that mediate the partitioning of black carbon (BC) and brown carbon (BrC) formation, as well as the spatial and temporal factors that drive particle evolution, are not understood adequately for many climate and air-quality related modeling applications. In situ observations provide considerable detail about aerosol microphysical and chemical properties, although sampling is extremely limited. Satellites offer the frequent global coverage that would allow for statistical characterization of emitted and evolved smoke, but generally lack microphysical detail. However, once properly validated, data from the National Aeronautics and Space Administration (NASA) Earth Observing System’s Multi-Angle Imaging Spectroradiometer (MISR) instrument can create at least a partial picture of smoke particle properties and plume evolution. We use in situ data from the Department of Energy’s Biomass Burning Observation Project (BBOP) field campaign to assess the strengths and limitations of smoke particle retrieval results from the MISR Research Aerosol (RA) retrieval algorithm. We then use MISR to characterize wildfire smoke particle properties and to identify the relevant aging factors in several cases, to the extent possible. The RA successfully maps qualitative changes in effective particle size, light absorption, and its spectral dependence, when compared to in situ observations. By observing the entire plume uniformly, the satellite data can be interpreted in terms of smoke plume evolution, including size-selective deposition, new-particle formation, and locations within the plume where BC or BrC dominates.
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    Wildfire Smoke Particle Properties and Evolution, From Space-Based Multi-Angle Imaging II: The Williams Flats Fire during the FIREX-AQ Campaign
    (MDPI, 2020-11-21) Junghenn Noyes, Katherine T.; Kahn, Ralph A.; Limbacher, James A.; Li, Zhanqing; Fenn, Marta A.; Giles, David M.; Hair, Johnathan W.; Katich, Joseph M.; Moore, Richard H.; Robinson, Claire E.; Sanchez, Kevin J.; Shingler, Taylor J.; Thornhill, Kenneth L.; Wiggins, Elizabeth B.; Winstead, Edward L.
    Although the characteristics of biomass burning events and the ambient ecosystem determine emitted smoke composition, the conditions that modulate the partitioning of black carbon (BC) and brown carbon (BrC) formation are not well understood, nor are the spatial or temporal frequency of factors driving smoke particle evolution, such as hydration, coagulation, and oxidation, all of which impact smoke radiative forcing. In situ data from surface observation sites and aircraft field campaigns offer deep insight into the optical, chemical, and microphysical traits of biomass burning (BB) smoke aerosols, such as single scattering albedo (SSA) and size distribution, but cannot by themselves provide robust statistical characterization of both emitted and evolved particles. Data from the NASA Earth Observing System’s Multi-Angle Imaging SpectroRadiometer (MISR) instrument can provide at least a partial picture of BB particle properties and their evolution downwind, once properly validated. Here we use in situ data from the joint NOAA/NASA 2019 Fire Influence on Regional to Global Environments Experiment-Air Quality (FIREX-AQ) field campaign to assess the strengths and limitations of MISR-derived constraints on particle size, shape, light-absorption, and its spectral slope, as well as plume height and associated wind vectors. Based on the satellite observations, we also offer inferences about aging mechanisms effecting downwind particle evolution, such as gravitational settling, oxidation, secondary particle formation, and the combination of particle aggregation and condensational growth. This work builds upon our previous study, adding confidence to our interpretation of the remote-sensing data based on an expanded suite of in situ measurements for validation. The satellite and in situ measurements offer similar characterizations of particle property evolution as a function of smoke age for the 06 August Williams Flats Fire, and most of the key differences in particle size and absorption can be attributed to differences in sampling and changes in the plume geometry between sampling times. Whereas the aircraft data provide validation for the MISR retrievals, the satellite data offer a spatially continuous mapping of particle properties over the plume, which helps identify trends in particle property downwind evolution that are ambiguous in the sparsely sampled aircraft transects. The MISR data record is more than two decades long, offering future opportunities to study regional wildfire plume behavior statistically, where aircraft data are limited or entirely lacking.
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    Satellite Remote Sensing of Smoke Particle Optical Properties, Their Evolution and Controlling Factors
    (2021) Junghenn, Katherine Teresa; Li, Zhanqing; Kahn, Ralph A.; Atmospheric and Oceanic Sciences; Digital Repository at the University of Maryland; University of Maryland (College Park, Md.)
    The optical and chemical properties of biomass burning (BB) smoke particles greatly affect the impact wildfires have on climate and air quality. Previous work has demonstrated some links between smoke properties and factors such as fuel type and meteorology. However, the factors controlling BB particle speciation at emission are not adequately understood, nor are those driving particle aging during atmospheric transport. As such, modeling wildfire smoke impacts on climate and air quality remains challenging. The potential to provide robust, statistical characterizations of BB particles based on ecosystem and ambient conditions with remote sensing data is investigated here. Space-based Multi-angle Imaging Spectrometer (MISR) observations, combined with the MISR Research Aerosol (RA) algorithm and the MISR Interactive Explorer (MINX) tool, are used to retrieve smoke plume aerosol optical depth (AOD), and to provide constraints on plume vertical extent, smoke age, and particle size, shape, light-absorption, and absorption spectral dependence. These capabilities are evaluated using near-coincident in situ data from two aircraft field campaigns. Results indicate that the satellite retrievals successfully map particle-type distributions, and that the observed trends in retrieved particle size and light-absorption can be reliably attributed to aging processes such as gravitational settling, oxidation, secondary particle formation, and condensational growth. The remote-sensing methods are then applied to numerous wildfire plumes in Canada and Alaska that are not constrained by field observations. For these plumes, satellite measurements of fire radiative power and land cover characteristics are also collected, as well as short-term meteorological data and drought index. We find statistically significant differences in the retrieved smoke properties based on land cover type, with fires in forests producing the tallest and thickest plumes containing the largest, brightest particles, and fires in savannas and grasslands exhibiting the opposite. Additionally, the inferred dominant aging mechanisms and the timescales over which they occur vary between land types. This work demonstrates the potential of remote sensing to constrain BB particle properties and the mechanisms governing their evolution, over entire ecosystems. It also begins to realize this potential, as a means of improving regional and global climate and air quality modeling in a rapidly changing world.