Theses and Dissertations from UMD

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    CHARACTERIZING RICE RESIDUE BURNING AND ASSOCIATED EMISSIONS IN VIETNAM USING A REMOTE SENSING AND FIELD-BASED APPROACH
    (2018) Lasko, Kristofer; Justice, Christopher O; Geography; Digital Repository at the University of Maryland; University of Maryland (College Park, Md.)
    Agricultural residue burning, practiced in croplands throughout the world, adversely impacts public health and regional air quality. Monitoring and quantifying agricultural residue burning with remote sensing alone is difficult due to lack of field data, hazy conditions obstructing satellite remote sensing imagery, small field sizes, and active field management. This dissertation highlights the uncertainties, discrepancies, and underestimation of agricultural residue burning emissions in a small-holder agriculturalist region, while also developing methods for improved bottom-up quantification of residue burning and associated emissions impacts, by employing a field and remote sensing-based approach. The underestimation in biomass burning emissions from rice residue, the fibrous plant material left in the field after harvest and subjected to burning, represents the starting point for this research, which is conducted in a small-holder agricultural landscape of Vietnam. This dissertation quantifies improved bottom-up air pollution emissions estimates through refinements to each component of the fine-particulate matter emissions equation, including the use of synthetic aperture radar timeseries to explore rice land area variation between different datasets and for date of burn estimates, development of a new field method to estimate both rice straw and stubble biomass, and also improvements to emissions quantification through the use of burning practice specific emission factors and combustion factors. Moreover, the relative contribution of residue burning emissions to combustion sources was quantified, demonstrating emissions are higher than previously estimated, increasing the importance for mitigation. The dissertation further explored air pollution impacts from rice residue burning in Hanoi, Vietnam through trajectory modelling and synoptic meteorology patterns, as well as timeseries of satellite air pollution and reanalysis datasets. The results highlight the inherent difficulty to capture air pollution impacts in the region, especially attributed to cloud cover obstructing optical satellite observations of episodic biomass burning. Overall, this dissertation found that a prominent satellite-based emissions dataset vastly underestimates emissions from rice residue burning. Recommendations for future work highlight the importance for these datasets to account for crop and burning practice specific emission factors for improved emissions estimates, which are useful to more accurately highlight the importance of reducing emissions from residue burning to alleviate air quality issues.
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    Photochemistry and transport of tropospheric ozone and its precursors in urban and remote environments
    (2016) Anderson, Daniel Craig; Dickerson, Russell R; Salawitch, Ross J; Atmospheric and Oceanic Sciences; Digital Repository at the University of Maryland; University of Maryland (College Park, Md.)
    Tropospheric ozone (O3) adversely affects human health, reduces crop yields, and contributes to climate forcing. To limit these effects, the processes controlling O3 abundance as well as that of its precursor molecules must be fully characterized. Here, I examine three facets of O3 production, both in heavily polluted and remote environments. First, using in situ observations from the DISCOVER-AQ field campaign in the Baltimore/Washington region, I evaluate the emissions of the O3 precursors CO and NOx (NOx = NO + NO2) in the National Emissions Inventory (NEI). I find that CO/NOx emissions ratios derived from observations are 21% higher than those predicted by the NEI. Comparisons to output from the CMAQ model suggest that CO in the NEI is accurate within 15 ± 11%, while NOx emissions are overestimated by 51-70%, likely due to errors in mobile sources. These results imply that ambient ozone concentrations will respond more efficiently to NOx controls than current models suggest. I then investigate the source of high O3 and low H2O structures in the Tropical Western Pacific (TWP). A combination of in situ observations, satellite data, and models show that the high O3 results from photochemical production in biomass burning plumes from fires in tropical Southeast Asia and Central Africa; the low relative humidity results from large-scale descent in the tropics. Because these structures have frequently been attributed to mid-latitude pollution, biomass burning in the tropics likely contributes more to the radiative forcing of climate than previously believed. Finally, I evaluate the processes controlling formaldehyde (HCHO) in the TWP. Convective transport of near surface HCHO leads to a 33% increase in upper tropospheric HCHO mixing ratios; convection also likely increases upper tropospheric CH3OOH to ~230 pptv, enough to maintain background HCHO at ~75 pptv. The long-range transport of polluted air, with NO four times the convectively controlled background, intensifies the conversion of HO2 to OH, increasing OH by a factor of 1.4. Comparisons between the global chemistry model CAM-Chem and observations show that consistent underestimates of HCHO by CAM-Chem throughout the troposphere result from underestimates in both NO and acetaldehyde.
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    AN APPROACH TO ESTIMATE GLOBAL BIOMASS BURNING EMISSIONS OF ORGANIC AND BLACK CARBON FROM MODIS FIRE RADIATIVE POWER
    (2009) Ellicott, Evan Andrew; Justice, Christopher O; Vermote, Eric; Geography; Digital Repository at the University of Maryland; University of Maryland (College Park, Md.)
    Biomass burning is an important global phenomenon affecting atmospheric composition with significant implications for climatic forcing. Wildland fire is the main global source of fine primary carbonaceous aerosols in the form of organic carbon (OC) and black carbon (BC), but uncertainty in aerosol emission estimates from biomass burning is still rather large. Application of satellite based measures of fire radiative power (FRP) has been demonstrated to offer an alternative approach to estimate biomass consumed with the potential to estimate the associated emissions from fires. To date, though, no study has derived integrated FRP (referred to as fire radiative energy or FRE) at a global scale, in part due to limitations in temporal or spatial resolution of satellite sensors. The main objective of this research was to quantify global biomass burning emissions of organic and black carbon aerosols and the corresponding effect on planetary radiative forcing. The approach is based on the geophysical relationship between the flux of FRE emitted, biomass consumed, and aerosol emissions. Aqua and Terra MODIS observations were used to estimate FRE using a simple model to parameterize the fire diurnal cycle based on the long term ratio between Terra and Aqua MODIS FRP and cases of diurnal satellite measurements of FRP made by the geostationary sensor SEVIRI, precessing sensor VIRS, and high latitude (and thus high overpass frequency) observations by MODIS. Investigation of the atmospheric attenuation of MODIS channels using a parametric model based on the MODTRAN radiative transfer model indicates a small bias in FRE estimates which was accounted for. Accuracy assessment shows that the FRE estimates are precise (R2 = 0.85), but may be underestimated. Global estimates of FRE show that Africa and South America dominate biomass burning, accounting for nearly 70% of the annual FRE generated. The relationship between FRE and OCBC estimates made with a new MODIS-derived inversion product of daily integrated biomass burning aerosol emissions was explored. The slope of the relationship within each of several biomes yielded a FRE-based emission factor. The biome specific emission factors and FRE monthly data were used to estimate OCBC emissions from fires on a global basis for 2001 to 2007. The annual average was 17.23 Tg which was comparable to previously published values, but slightly lower. The result in terms of global radiative forcing suggests a cooling effect at both the top-of-atmosphere (TOA) and surface approaching almost -0.5 K which implies that biomass burning aerosols could dampen the warming effect of green house gas emissions. An error budget was developed to explore the sources and total uncertainty in the OCBC estimation. The results yielded an uncertainty value of 58% with specific components of the process warranting future consideration and improvement. The uncertainty estimate does not demonstrate a significant improvement over current methods to estimate biomass burning aerosols, but given the simplicity of the approach should allow for refinements to be made with relative ease.
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    Detection, Evaluation, and Analysis of Global Fire Activity Using MODIS Data
    (2006-04-26) Giglio, Louis; Justice, Christopher O; Geography; Digital Repository at the University of Maryland; University of Maryland (College Park, Md.)
    Global biomass burning plays a significant role in regional and global climate change, and spaceborne sensors offer the only practical way to monitor fire activity at these scales. This dissertation primarily concerns the development, evaluation, and use of the NASA Terra and Aqua MODIS instruments for fire monitoring. MODIS is the first satellite sensor designed specifically for global monitoring of fires. An improved operational fire detection algorithm was developed for the MODIS instrument. This algorithm offers a sensitivity to small, cool fires and minimizes false alarm rates. To support the accuracy assessment of the MODIS global fire product, an operational fire detection algorithm was developed and evaluated for the ASTER instrument, which provides higher resolution observations coincident with the Terra MODIS. The unique data set of multi-year MODIS day and night fire observations was used to analyze the global distribution of biomass burning using five different temporal metrics which included, for the first time, mean fire radiative power, a measure of fire intensity. The metrics show the planetary extent, seasonality, and interannual variability of fire. Recognizing differences in fire activity between morning and afternoon overpasses, the impact of the diurnal cycle of fire activity was addressed using seven years of fire data from the VIRS sensor on-board the TRMM satellite. A strong diurnal cycle was found in all regions, with the time of peak burning varying between approximately 13:00 and 18:30 local time. Given interest in area burned among atmospheric chemical transport and carbon cycle modelers, a data set was developed utilizing the MODIS global fire and vegetation cover products to estimate monthly burned area at 1-degree spatial resolution. The methods, products and results presented in this thesis provide the global change research and fire management communities with products for global fire monitoring and are currently being used in the development of the next generation of operational satellite fire monitoring systems.
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    MODELING OF SEASONAL TRACE GAS AND PARTICULATE EMISSIONS FROM VEGETATION FIRES IN SOUTHERN AFRICA
    (2004-04-29) Korontzi, Stefania; Justice, Christopher O; Geography
    Fire is widespread in southern African savannas with important implications for tropical and global atmospheric chemistry. However, previous regional emission studies have not fully accounted for the variability of the emissions throughout the burning season and the associated impacts on emissions quantification. The main aim of this study is to address this gap. The complexity of the emissions process is described using a spatially and temporally explicit modeling approach that integrates recently published satellite-driven fuel load amounts, satellite burned area products, and empirically derived parameterizations of combustion completeness and emission factors. To represent fire behavior characteristics, land cover is classified into grasslands and woodlands, using a satellite-derived percent tree cover product. The combustion completeness is modeled as a function of grass fuel moisture and the emission factors as a function of grass fuel moisture in grasslands and fuel mixture in woodlands. Fuel moisture is derived from a fuel load model and by using satellite vegetation index time series. A sensitivity analysis with respect to three satellite burned area products reveals large differences in emissions due to differences in their amounts and spatial distribution. The analysis at the regional scale shows, that early burning in grasslands may lead to higher amounts of products of incomplete combustion despite the lower amounts of fuel consumed, compared with late dry season burning. In contrast, early burning in woodlands results in lower emissions because less fuel gets consumed. These seasonal emissions trends become more pronounced when the fuels are wetter. Burning in woodlands dominates the regional emissions budgets. Emissions estimates for various atmospheric species, many of which are modeled for the first time, are reported and compared with other regional sources of pyrogenic emissions and global biomass burning and fossil fuel emissions. The modeled estimates for 2000 are (in Tg): 537 CO<sub>2</sub>, 23.2 CO, 0.726 CH<sub>4</sub>, 0.661 NMHC, 2.4 particulates (< 2.5 micron), 1.0 NO<sub>x</sub> and account for significant fractions of regional emissions from all pyrogenic sources. Especially high is the previously undetermined contribution of Oxygenated Volatile Organic Compounds (1.8 Tg). The methodology and results have direct implications for national reporting of savanna fire emissions.