Theses and Dissertations from UMD
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Item Optical properties of a quantum-noise-limited phase-sensitive amplifier(2017) Li, Tian; Lett, Paul D.; Rolston, Steven L.; Physics; Digital Repository at the University of Maryland; University of Maryland (College Park, Md.)This dissertation is a summary of investigations on the optical properties of a quantum-noise-limited phase-sensitive amplifier (PSA). The PSA is implemented using four-wave mixing in hot Rb 85 vapor based on a double-Lambda atomic scheme. We experimentally demonstrate the ability of a PSA to pre-amplify quantum correlations in twin light beams produced by a phase-insensitive amplifier (PIA) before degradation due to loss and detector inefficiency. By including a PSA before loss, one is able to preserve the correlations as well as the two-mode squeezing level. We compare the results to simulations employing a simple quantum-mechanical model and find a good agreement. We have demonstrated that the cross-correlation between the two modes of a bipartite entangled state can be advanced by propagation through a PIA acting as a fast-light medium. The extra noise added by the PIA has been speculated to be the mechanism that limits the advance of entanglement, preventing the mutual information from traveling superluminally. As an extension of this phase-insensitive, gain-assisted, anomalous dispersion investigation, we explore the advance and delay of information transmitted through the PSA. We start with a two-mode squeezed state created by the PIA and measure the mutual information shared by the correlated quadratures. We then pass one of these two modes through a PSA and investigate the shift of the mutual information as a function of the PSA phase. In the case of a PSA, it is well known that no extra noise will be added to the quadrature with the correct input phase (e.g., the quadrature with the maximal amplification or the maximal deamplification). We find that there is no dispersion-like behavior at these two phases, however, the peak of mutual information could either be delayed or advanced at any other phase. We also observe an almost identical behavior when we input an amplitude modulated signal to the PSA. We are able to explain the physics of this ``fast-and-slow-light'' type of behavior utilizing a model assuming imbalanced gain on the positive and negative side bands. We obtain a good agreement between the experimental results and the theoretical simulations.Item Self-Assembled InAs/GaAs Quantum Dot Solar Cells(2015) Li, Tian; Dagenais, Mario; Electrical Engineering; Digital Repository at the University of Maryland; University of Maryland (College Park, Md.)Our work focuses on experimental and theoretical studies aimed at establishing a fundamental understanding of the principal electrical and optical processes governing the operation of quantum dot solar cells (QDSC) and their feasibility for the realization of intermediate band solar cell (IBSC). Uniform performance QD solar cells with high conversion efficiency have been fabricated using carefully calibrated process recipes as the basis of all reliable experimental characterization. The origin for the enhancement of the short circuit current density (Jsc) in QD solar cells was carefully investigated. External quantum efficiency (EQE) measurements were performed as a measure of the below bandgap distribution of transition states. In this work, we found that the incorporation of self-assembled quantum dots (QDs) interrupts the lattice periodicity and introduce a greatly broadened tailing density of states extending from the bandedge towards mid-gap. A below-bandgap density of states (DOS) model with an extended Urbach tail has been developed. In particular, the below-bandgap photocurrent generation has been attributed to transitions via confined energy states and background continuum tailing states. Photoluminescence measurement is used to measure the energy level of the lowest available state and the coupling effect between QD states and background tailing states because it results from a non-equilibrium process. A basic I-V measurement reveals a degradation of the open circuit voltage (Voc) of QD solar cells, which is related to a one sub-bandgap photon absorption process followed by a direct collection of the generated carriers by the external circuit. We have proposed a modified Shockley-Queisser (SQ) model that predicts the degradation of Voc compared with a reference bulk device. Whenever an energy state within the forbidden gap can facilitate additional absorption, it can facilitate recombination as well. If the recombination is non-radiative, it is detrimental to solar cell performance. We have also investigated the QD trapping effects as deep level energy states. Without an efficient carrier extraction pathway, the QDs can indeed function as mobile carriers traps. Since hole energy levels are mostly connected with hole collection under room temperature, the trapping effect is more severe for electrons. We have tried to electron-dope the QDs to exert a repulsive Coulomb force to help improve the carrier collection efficiency. We have experimentally observed a 30% improvement of Jsc for 4e/dot devices compared with 0e/dot devices. Electron-doping helps with better carrier collection efficiency, however, we have also measured a smaller transition probability from valance band to QD states as a direct manifestation of the Pauli Exclusion Principle. The non-linear performance is of particular interest. With the availability of laser with on-resonance and off-resonance excitation energy, we have explored the photocurrent enhancement by a sequential two-photon absorption (2PA) process via the intermediate states. For the first time, we are able to distinguish the nonlinearity effect by 1PA and 2PA process. The observed 2PA current under off-resonant and on-resonant excitation comes from a two-step transition via the tailing states instead of the QD states. However, given the existence of an extended Urbach tail and the small number of photons available for the intermediate states to conduction band transition, the experimental results suggest that with the current material system, the intensity requirement for an observable enhancement of photocurrent via a 2PA process is much higher than what is available from concentrated sun light. In order to realize the IBSC model, a matching transition strength needs to be achieved between valance band to QD states and QD states to conduction band. However, we have experimentally shown that only a negligible amount of signal can be observed at cryogenic temperature via the transition from QD states to conduction band under a broadband IR source excitation. Based on the understanding we have achieved, we found that the existence of the extended tailing density of states together with the large mismatch of the transition strength from VB to QD and from QD to CB, has systematically put into question the feasibility of the IBSC model with QDs.