Atmospheric & Oceanic Science Theses and Dissertations
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Browsing Atmospheric & Oceanic Science Theses and Dissertations by Subject "aerosols"
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Item AN INVESTIGATION OF CIRRUS CLOUD PROPERTIES USING AIRBORNE LIDAR(2014) Yorks, John E.; Dickerson, Russell R; McGill, Matthew J; Atmospheric and Oceanic Sciences; Digital Repository at the University of Maryland; University of Maryland (College Park, Md.)The impact of cirrus clouds on the Earth's radiation budget remains a key uncertainty in assessing global radiative balance and climate change. Composed of ice, and located in the cold upper troposphere, cirrus clouds can cause large warming effects because they are relatively transmissive to short-wave solar radiation, but absorptive of long wave radiation. Our ability to model radiative effects of cirrus clouds is inhibited by uncertainties in cloud optical properties. Studies of mid-latitude cirrus properties have revealed notable differences compared to tropical anvil cirrus, likely a consequence of varying dynamic formation mechanisms. Cloud-aerosol lidars provide critical information about the vertical structure of cirrus for climate studies. For this dissertation, I helped develop the Airborne Cloud-Aerosol Transport System (ACATS), a Doppler wind lidar system at NASA Goddard Space Flight Center (GSFC). ACATS is also a high spectral resolution lidar (HSRL), uniquely capable of directly resolving backscatter and extinction properties of a particle from high-altitude aircraft. The first ACATS science flights were conducted out of Wallops Island, VA in September of 2012 and included coincident measurements with the Cloud Physics Lidar (CPL) instrument. In this dissertation, I provide an overview of the ACATS method and instrument design, describe the ACATS retrieval algorithms for cloud and aerosol properties, explain the ACATS HSRL retrieval errors due to the instrument calibration, and use the coincident CPL data to validate and evaluate ACATS cloud and aerosol retrievals. Both the ACATS HSRL and standard backscatter retrievals agree well with coincident CPL retrievals. Mean ACATS and CPL extinction profiles for three case studies demonstrate similar structure and agree to within 25 percent for cirrus clouds. The new HSRL retrieval algorithms developed for ACATS have direct application to future spaceborne missions. Furthermore, extinction and particle wind velocity retrieved from ACATS can be used for science applications such as dust transport and convective anvil outflow. The relationship between cirrus cloud properties and dynamic formation mechanism is examined through statistics of CPL cirrus observations from more than 100 aircraft flights. The CPL 532 nm lidar ratios (also referred to as the extinction to backscatter ratio) for cirrus clouds formed by synoptic-scale uplift over land are lower than convectively-generated cirrus over tropical oceans. Errors in assuming a constant lidar ratio can lead to errors of ~50% in cloud optical extinction derived from space-borne lidar such as CALIOP. The 1064 nm depolarization ratios for synoptically-generated cirrus over land are lower than convectively-generated cirrus, formed due to rapid upward motions of tropical convection, as a consequence of differences in cloud temperatures and ice particle size and shape. Finally, the backscatter color ratio is directly proportional to depolarization ratio for synoptically-generated cirrus, but not for any other type of cirrus. The relationships between cirrus properties and formation mechanisms determined in this study can be used as part of a larger global climatology of cirrus clouds to improve parameterizations in global climate models and satellite retrievals to improve our understanding of the impact of clouds on weather and climate.Item Multi-sensor Cloud and Aerosol Retrieval Simulator and Its Applications(2016) Wind, Galina; Salawitch, Ross J; Platnick, Steven; Atmospheric and Oceanic Sciences; Digital Repository at the University of Maryland; University of Maryland (College Park, Md.)Executing a cloud or aerosol physical properties retrieval algorithm from controlled synthetic data is an important step in retrieval algorithm development. Synthetic data can help answer questions about the sensitivity and performance of the algorithm or aid in determining how an existing retrieval algorithm may perform with a planned sensor. Synthetic data can also help in solving issues that may have surfaced in the retrieval results. Synthetic data become very important when other validation methods, such as field campaigns,are of limited scope. These tend to be of relatively short duration and often are costly. Ground stations have limited spatial coverage whilesynthetic data can cover large spatial and temporal scales and a wide variety of conditions at a low cost. In this work I develop an advanced cloud and aerosol retrieval simulator for the MODIS instrument, also known as Multi-sensor Cloud and Aerosol Retrieval Simulator (MCARS). In a close collaboration with the modeling community I have seamlessly combined the GEOS-5 global climate model with the DISORT radiative transfer code, widely used by the remote sensing community, with the observations from the MODIS instrument to create the simulator. With the MCARS simulator it was then possible to solve the long standing issue with the MODIS aerosol optical depth retrievals that had a low bias for smoke aerosols. MODIS aerosol retrieval did not account for effects of humidity on smoke aerosols. The MCARS simulator also revealed an issue that has not been recognized previously, namely,the value of fine mode fraction could create a linear dependence between retrieved aerosol optical depth and land surface reflectance. MCARS provided the ability to examine aerosol retrievals against “ground truth” for hundreds of thousands of simultaneous samples for an area covered by only three AERONET ground stations. Findings from MCARS are already being used to improve the performance of operational MODIS aerosol properties retrieval algorithms. The modeling community will use the MCARS data to create new parameterizations for aerosol properties as a function of properties of the atmospheric column and gain the ability to correct any assimilated retrieval data that may display similar dependencies in comparisons with ground measurements.Item A STUDY OF OPTICAL, PHYSICAL AND CHEMICAL PROPERTIES OF AEROSOLS USING IN SITU MEASUREMENTS(2009) Chaudhry, Zahra; Li, Zhanqing; Atmospheric and Oceanic Sciences; Digital Repository at the University of Maryland; University of Maryland (College Park, Md.)Using a simple sampling apparatus, aerosol particles were collected on a polycarbonate substrate in various locations around the world. The focus of this study was Xianghe, China, an industrial town 70 km southeast of Beijing. The Nuclepore filters were collected in two size ranges (coarse, 2.5μm < d < 10μm, and fine, d < 2.5μm) from January-December 2005, with a focus on the Intensive Observation Campaign (IOC) in March 2005. The collected filters were analyzed for aerosol mass concentration and aerosol absorption efficiency; selected filters were analyzed for chemical composition. For fine mode aerosols measured during the Xianghe 2005 IOC, the average spectral absorption efficiency equates well to a &lamda;-1 model, while the coarse mode shows a much flatter spectral dependence, consistent with large particle models. The coarse mode absorption efficiency was compatible with that of the fine mode in the near-IR region, indicating the much stronger absorption of the coarse mode due to its composition and sizeable mass. Ground-based measurements were compared to remote sensing instruments that measure similar parameters for the total column. A co-located lidar assisted in determination of vertical homogeneity. For cases of vertical homogeneity, the ground-based measurements were able to represent total column measurements well. For cases of vertical inhomogeneity, ground-based measurements did not equate well to total column measurements. The layers of aerosols that form in the atmosphere have significant effects on the temperature profile. An instrument was developed to measure aerosol absorption and scattering, the Scattering and Absorption Sonde (SAS). This instrument was launched seven times at two locations in China in 2008. Vertical profiles of scattering coefficient were measured and several aerosol layers were identified. The aerosol characterized at Xianghe, China was compared to aerosol characteristics from Kanpur, India and Mexico City, Mexico. The aerosol at Mexico City differs greatly from that at Xianghe, based on the measured mass concentration, aerosol size distribution from AERONET, and measured aerosol absorption efficiency. The aerosol at Kanpur resembles well the aerosol characterized at Xianghe in the fine mode, with a correlation of 0.998 for the aerosol absorption efficiency.