Theses and Dissertations from UMD
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New submissions to the thesis/dissertation collections are added automatically as they are received from the Graduate School. Currently, the Graduate School deposits all theses and dissertations from a given semester after the official graduation date. This means that there may be up to a 4 month delay in the appearance of a give thesis/dissertation in DRUM
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Item HIGH THROUGHPUT STIMULATED BRILLOUIN SCATTERING SPECTROSCOPY(2024) Rosvold, Jake Robert; Scarcelli, Giuliano; Bioengineering; Digital Repository at the University of Maryland; University of Maryland (College Park, Md.)Brillouin light scattering arises from the coupled interaction between light and material acoustic phonons. The measurand of Brillouin scattering is the characteristic frequency difference between incident and scattered light which depends on the local longitudinal modulus of the material. Spontaneous Brillouin scattering has been used in combination with confocal microscopy to provide non-contact, label-free mapping at micron-scale resolution in biological media. To date, spontaneous Brillouin microscopy has reached the speed limit (~20-50ms per spectrum) as determined by the theoretical scattering efficiency. While a great deal of research has been directed to speeding up Brillouin microscopy acquisition times, spontaneous Brillouin scattering is fundamentally an inefficient process thus limiting the ability to study faster biological phenomena and rapid processes. To combat this limitation, its nonlinear counterpart, stimulated Brillouin scattering (SBS) has been proposed for microscopy applications. For decades, stimulated Brillouin scattering has been used in fiber sensing and all-optical pulse control and leverages a nonlinear interaction where two counterpropagating light beams stimulate a more efficient scattering relationship. However, the small interaction volumes and photodamage constraints presented in microscopy have hindered the translation of stimulated Brillouin scattering into the biological realm. Recently, continuous wave stimulated Brillouin microscopy has led to competitive acquisition times (~5ms per spectrum) when compared to the spontaneous alternative but has yet to be widely adopted. Due to a plethora of factors, such as an inefficient power balance between pump and probe beams, lack of proper commercial laser sources, and nonoptimal detection schemes, the complete picture of what SBS spectroscopy has to offer has yet to be revealed. As such, there is a need to customize light sources and detection schemes in order to fully take advantage of the enhanced Brillouin efficiency possible in SBS. Herein we introduce novel methodology to improve the acquisition speed of Brillouin microscopy by designing and developing proper laser sources and detection schemes for efficient SBS spectroscopy. First, we showcase the potential utility of our state-of-the-art continuous wave SBS technology in a flow cytometry application, highly suitable for the counterpropagating geometry of SBS where the laser position is fixed while the sample is being moved at high speeds. Additionally, we will present an optimized receiver design based on polarization detection which enables 100x faster spectral measurements in the low-gain regime relevant to biological materials. Finally, we demonstrate an optimal pulsed laser source specifically designed for SBS Brillouin microscopy.Item NONLINEAR PROPAGATION OF ORBITAL ANGULAR MOMENTUM LIGHT IN TURBULENCE AND FIBER(2024) Elder, Henry; Sprangle, Phillip; Physics; Digital Repository at the University of Maryland; University of Maryland (College Park, Md.)Light that carries orbital angular momentum (OAM), also referred to as optical vortices or twisted light, is characterized by a helical or twisted wavefront ∝exp[imφ]. In contrast to spin angular momentum (SAM), where photons are limited to two states, OAM allows for, in principle, an infinite set of spatially orthogonal states. OAM-carrying light has found applications ranging from quantum key distribution in free space and guided-wave communication systems, particle trapping and optical tweezers, nanoscopy, and remote sensing. Understanding how OAM light propagates through complex environments, and how to efficiently generate particular OAM states, is critical for any such application. In the first part of this dissertation, we describe how OAM light propagates through a turbulent atmosphere. We build analytic models which describe (1) the OAM mode mixing caused by turbulence, (2) the evolution of short, high-power OAM pulses undergoing the effects of self-phase modulation (SPM) and group velocity dispersion (GVD), and (3) the evolution of high-power Gaussian pulses including SPM, GVD, and turbulence. The models are validated against both experimental data and nonlinear, turbulent pulse propagation simulation programs, the latter of which we have made freely available. We also explore how self-focusing can minimize certain deleterious effects of turbulence for OAM light. The second part of this dissertation considers nonlinear effects of OAM light propagating in azimuthally symmetric waveguides. Such waveguides have so-called spin-orbit (SO) modes, which are quantized based on their total angular momentum (TAM). We develop a generalized theory of four wave mixing-based parametric amplification of SO modes and show that these processes conserve TAM, but under certain circumstances can be taken to conserve SAM and OAM independently. Our theory is validated against a nonlinear multimode beam propagation simulation program which we developed and, again, have made freely available.Item Spatiotemporal Optical Vortices(2023) Hancock, Scott; Milchberg, Howard; Physics; Digital Repository at the University of Maryland; University of Maryland (College Park, Md.)Light beams carrying orbital angular momentum (OAM) have become a mainstay of optical science and technology. In these beams, well-known examples of which are the Laguerre-Gaussian (LG_pm ) and Bessel-Gaussian (BG_m ) beams, the OAM vector points parallel or anti-parallel to propagation, and is associated with a phase winding 2πm in the plane transverse to the propagation direction, where integer m is the winding order or the “topological charge”. Such beams can be monochromatic.Recently, our group discovered a new type of OAM structure that naturally emerges from nonlinear self-focusing, which we dubbed the spatio-temporal optical vortex (STOV). Here, the phase winding exists in a spatiotemporal plane, with the OAM pointing transverse to propagation. In this dissertation, we extend the generation of STOV-carrying pulses to the linear regime, demonstrating their generation using a 4f pulse shaper and measuring their free-space propagation using a new ultrafast single-shot space- and time-resolving diagnostic, TG-SSSI (transient-grating single-shot supercontinuum spectral interferometry). We then demonstrate that transverse OAM is a property of photons by experimentally confirming the conservation of transverse OAM in second harmonic generation. Because the field of STOVs is so new, a first principles theory for their transverse OAM was lacking. We developed such a theory for transverse OAM that predicts half integer values of OAM and the existence of a STOV polariton in dispersive media. The surprise of half-integer OAM values launched a debate in the OAM community, which has been resolved in favor of our theory by our most recent experiments. These explore how phase and amplitude perturbations can impart spatiotemporal torques to light. We find that transverse OAM can be imparted to light pulses only for (1) sufficiently fast transient phase perturbations or (2) energy removal from a pulse already possessing transverse OAM.Item QUANTUM MODEM AND ROUTER FOR THE QUANTUM INTERNET(2022) Saha, Uday; Waks, Edo; Electrical Engineering; Digital Repository at the University of Maryland; University of Maryland (College Park, Md.)Like the internet, the quantum internet can change the world by connecting quantum computers over long distances. This connectivity can revolutionize different industries like banking, healthcare, and data analytics that utilize quantum computing and simulations. Additionally, it would enable us to connect multiple small quantum computers into powerful distributed quantum computers that can solve problems of significant societal impact. Despite the rise of excellent quantum computers, we don't yet have the core technologies to connect them. This is because modems and routers we use to connect classical computers don't work for quantum information. They destroy the coherence and entanglement of quantum information, which is vital for connecting quantum computers. In my thesis, I developed a quantum modem and router that can connect quantum computers and create a scalable quantum network. I have conceived the modem and router for the trapped ion quantum computers, the most promising quantum computing platform. However, we can easily use my developed concepts to connect different quantum computing platforms. I accomplished a quantum modem that provides an interface between a quantum computer and a fiber-optic network by generating telecommunication photons from the computer. I used a two-stage quantum frequency conversion scheme to realize the quantum modem. By calculating the second-order correlation function, I experimentally verified single-photon characteristics retained after the frequency conversion process. Telecommunication photons generated by the quantum modem can carry quantum information from ions over long distances. This will allow a long-distance quantum network to realize the quantum internet. On the other hand, I implemented a quantum router with photonic integrated circuits. Utilizing the thermo-optic property, I route photons from a trapped barium ion into different output ports of the quantum router in a programmable manner. This router can connect multiple quantum computers on-demand and in a scalable way. We are the first group to demonstrate a quantum modem and router working together with a quantum computer. This demonstration could lead to a scalable quantum network where photons from different quantum computers can be interfered with a programmable photonic chip to herald entanglement. Additionally, I developed visible photonic circuits for quantum data centers. In a quantum data center, there can be multiple trapped ion quantum computers that need to be connected. For this purpose, I designed a photonic circuit on a thin-film lithium niobate platform that can entangle two trapped ion quantum computers with >99% fidelity. Apart from achieving high fidelity entanglement, the circuit can achieve any polarization-independent power splitting ratio, which can have extensive use in integrated photonic technology. Finally, I invented a multiplexing scheme by which we can send quantum information from multiple quantum computers using a single fiber-optic cable. That will increase the channel capacity, where multiple quantum computers can communicate through the same channel. By encoding quantum information into the different wavelengths of photons, I devised my idea of multiplexing quantum information. These results will enable us to achieve a programmable and scalable network of quantum computers to increase the capability of quantum computing and quantum simulations and lead us to the future quantum internet.Item Experiments with Frequency Converted Photons from a Trapped Atomic Ion(2022) Hannegan, John Michael; Quraishi, Qudsia; Linke, Norbert; Physics; Digital Repository at the University of Maryland; University of Maryland (College Park, Md.)Trapped atomic ions excel as local quantum information processing nodes, given their long qubit coherence times combined with high fidelity single-qubit and multi-qubit gate operations. Trapped ion systems also readily emit photons as flying qubits, making efforts towards construction of large-scale and long-distance trapped-ion-based quantum networks very appealing. Two-node trapped-ion quantum networks have demonstrated a desirable combination of high-rate and high-fidelity remote entanglement generation, but these networks have been limited to only a few meters in length. This limitation is primarily due to large fiber-optic propagation losses experienced by the ultraviolet and visible photons typically emitted by trapped ions. These wavelengths are also incompatible with existing telecommunications technology and infrastructure, as well as being incompatible with many other emerging quantum technologies designed for useful tasks such as single photon storage, measurement, and routing, limiting the scalability of ion-based networks. In this thesis, I discuss a series of experiments where we introduce quantum frequency conversion to convert single photons at 493 nm, produced by and entangled with a single trapped $^{138}$Ba$^+$ ion, to near infrared wavelengths for reduced network transmission losses and improved quantum networking capabilities. This work is the first-ever to frequency convert Ba$^+$ photons, being one of three nearly concurrent demonstrations of frequency converted photons from any trapped ion. After discussing our experimental techniques and laboratory setup, I first showcase our quantum frequency converters that convert ion-produced single photons to both 780 nm and 1534 nm for improved quantum networking range, whilst preserving the photons' quantum properties. Following this, I present two hybrid quantum networking experiments where we interact converted ion-photons near 780 nm with neutral $^{87}$Rb systems. In the initial experiment, we observe, for the first time, interactions between converted ion-photons and neutral Rb vapor via slow light. The following experiment is a multi-laboratory project where we observe Hong-Ou-Mandel interference between converted ion-photons and photons produced by an ensemble of neutral Rb atoms, where notably these sources are located in different buildings and are connected and synchronized via optical fiber. Finally, I describe an experiment in which we verify entanglement between a $^{138}$Ba$^+$ ion and converted photons near 780 nm. These results are critical steps towards producing remote entanglement between trapped ion and neutral atom quantum networking nodes. Motivated by these experimental results, I conclude by presenting a theoretical hybrid-networking architecture where neutral-atomic based nondestructive single photon measurement and storage can be integrated into a long-distance trapped-ion based quantum network to potentially improve remote entanglement rates.Item Towards Low-frequency Squeezed Light and Its Applications with Four-wave Mixing in Rubidium Vapor(2020) Wu, Meng-Chang; Lett, Paul D.; Rolston, Steven L.; Chemical Physics; Digital Repository at the University of Maryland; University of Maryland (College Park, Md.)We study a variety of mechanisms that introduce noise into squeezed light generated by a four-wave mixing (4WM) process in Rb vapor. The noise from the seeding beam itself is a general noise that appears in any squeezed light generated from a seeding process. This noise dominates in the squeezed light at acoustic and lower measurement frequencies. A second excess noise source is observed in the twin beams pumped by either a diode laser system or a Ti:sapphire laser system. This excess noise is much stronger in the diode laser systems. It is present in the twin beams at measurement frequencies when the 4WM gain is reduced toward unity. Most of this excess noise can be removed with a dual-seeded 4WM scheme. A third noise source we examine is from a two-beam coupling that degrades the squeezing of the dual-seeded 4WM process at low frequencies of the order of the atomic transition linewidth. This noise can be avoided by seeding skew rays in the 4WM gain region. This gives us an insight to solve this "cross talk" problem by imaging the source in the 4WM gain region. In addition to studying noise sources, we propose a gain-independent calibration scheme that relies on higher order correlation function for the absolute calibration of photodiodes. Having low frequency squeezing is really important if we record quantum images with a CCD camera, which has a slow shutter speed. Also, it's been very difficult for people to get low-frequency squeezing. We obtain a record level of low-frequency squeezing using a simple dual-seeding technique. With this study of noise sources we are closer to having a portable quantum light source using diode lasers.Item Energy Deposition in Femtosecond Filamentation: Measurements and Applications(2017) Rosenthal, Eric Wieslander; Milchberg, Howard M; Physics; Digital Repository at the University of Maryland; University of Maryland (College Park, Md.)Femtosecond filamentation is a nonlinear optical propagation regime of high peak power ultrashort laser pulses characterized by an extended and narrow core region of high intensity whose length greatly exceeds the Rayleigh range corresponding to the core diameter. Providing that a threshold power is exceeded, filamentation can occur in all transparent gaseous, liquid and solid media. In air, filamentation has found a variety of uses, including the triggering of electric discharges, spectral broadening and compression of ultrashort laser pulses, coherent supercontinuum generation, filament-induced breakdown spectroscopy, generation of THz radiation, and the generation of air waveguides. Several of these applications depend on the deposition of energy in the atmosphere by the filament. The main channels for this deposition are the plasma generated in the filament core by the intense laser field and the rotational excitation of nitrogen and oxygen molecules. The ultrafast deposition acts as a delta function-like pressure source to drive a hydrodynamic response in the air. This thesis experimentally demonstrates two applications of the filament-driven hydrodynamic response. One application is the ‘air waveguide’, which is shown to either guide a separately injected laser pulse, or act as a remote collection optic for weak optical signals. The other application is the high voltage breakdown of air, where the effect of filament-induced plasmas and hydrodynamic response on the breakdown dynamics is elucidated in detail. In all of these experiments, it is important to understand quantitatively the laser energy absorption; detailed absorption experiments were performed as a function of laser parameters. Finally, as check on simulations of filament propagation and energy deposition, we measured the axially resolved energy deposition of a filament; in the simulations, this profile is quite sensitive to the choice of the nonlinear index of refraction (n2). We found that using our measured values of n2 in the propagation simulations results in an excellent fit to the measured energy deposition profiles.Item Nonlinear Optics and Carrier Dynamics in Nanostructured and Two-Dimensional Materials(2016) Suess, Ryan; Murphy, Thomas E; Electrical Engineering; Digital Repository at the University of Maryland; University of Maryland (College Park, Md.)Understanding and measuring the interaction of light with sub-wavelength structures and atomically thin materials is of critical importance for the development of next generation photonic devices. One approach to achieve the desired optical properties in a material is to manipulate its mesoscopic structure or its composition in order to affect the properties of the light-matter interaction. There has been tremendous recent interest in so called two-dimensional materials, consisting of only a single to a few layers of atoms arranged in a planar sheet. These materials have demonstrated great promise as a platform for studying unique phenomena arising from the low-dimensionality of the material and for developing new types of devices based on these effects. A thorough investigation of the optical and electronic properties of these new materials is essential to realizing their potential. In this work we present studies that explore the nonlinear optical properties and carrier dynamics in nanoporous silicon waveguides, two-dimensional graphite (graphene), and atomically thin black phosphorus. We first present an investigation of the nonlinear response of nanoporous silicon optical waveguides using a novel pump-probe method. A two-frequency heterodyne technique is developed in order to measure the pump-induced transient change in phase and intensity in a single measurement. The experimental data reveal a characteristic material response time and temporally resolved intensity and phase behavior matching a physical model dominated by free-carrier effects that are significantly stronger and faster than those observed in traditional silicon-based waveguides. These results shed light on the large optical nonlinearity observed in nanoporous silicon and demonstrate a new measurement technique for heterodyne pump-probe spectroscopy. Next we explore the optical properties of low-doped graphene in the terahertz spectral regime, where both intraband and interband effects play a significant role. Probing the graphene at intermediate photon energies enables the investigation of the nonlinear optical properties in the graphene as its electron system is heated by the intense pump pulse. By simultaneously measuring the reflected and transmitted terahertz light, a precise determination of the pump-induced change in absorption can be made. We observe that as the intensity of the terahertz radiation is increased, the optical properties of the graphene change from interband, semiconductor-like absorption, to a more metallic behavior with increased intraband processes. This transition reveals itself in our measurements as an increase in the terahertz transmission through the graphene at low fluence, followed by a decrease in transmission and the onset of a large, photo-induced reflection as fluence is increased. A hybrid optical-thermodynamic model successfully describes our observations and predicts this transition will persist across mid- and far-infrared frequencies. This study further demonstrates the important role that reflection plays since the absorption saturation intensity (an important figure of merit for graphene-based saturable absorbers) can be underestimated if only the transmitted light is considered. These findings are expected to contribute to the development of new optoelectronic devices designed to operate in the mid- and far-infrared frequency range. Lastly we discuss recent work with black phosphorus, a two-dimensional material that has recently attracted interest due to its high mobility and direct, configurable band gap (300 meV to 2eV), depending on the number of atomic layers comprising the sample. In this work we examine the pump-induced change in optical transmission of mechanically exfoliated black phosphorus flakes using a two-color optical pump-probe measurement. The time-resolved data reveal a fast pump-induced transparency accompanied by a slower absorption that we attribute to Pauli blocking and free-carrier absorption, respectively. Polarization studies show that these effects are also highly anisotropic - underscoring the importance of crystal orientation in the design of optical devices based on this material. We conclude our discussion of black phosphorus with a study that employs this material as the active element in a photoconductive detector capable of gigahertz class detection at room temperature for mid-infrared frequencies.