In this dissertation, we present new channels for the production of gravitational radiation sources: mergers of black holes in the nuclear star clusters found in many small galaxies, and mergers and tidal separations of black hole binaries in galaxies that host supermassive black holes. Mergers between stellar-mass black holes will be key sources of gravitational radiation for ground-based detectors. However, the rates of these events are highly uncertain, because we can not observe these binaries electromagnetically. In this work, we show that the nuclear star clusters found in the centers of small galaxies are conducive environments for black hole mergers. These clusters have large escape velocities, high stellar densities, and large numbers of black holes that will have multiple close encounters, which often lead to mergers. We present simulations of the three-body dynamics of black holes in this environment and estimate that, if many nuclear star clusters do not have supermassive black holes, tens of events per year will be detectable with Advanced LIGO. Larger galaxies that host supermassive black holes can produce extreme-mass ratio inspiral (EMRI) events, which are important sources for the future space-based detector, LISA. Here, we show that tidal separation of black hole binaries by supermassive black holes will produce a distinct class of EMRIs with near-zero eccentricities, and we estimate that rates from tidal separation could be comparable to or larger than those from the traditionally-discussed two-body capture formation scenario. Before tidal separation can occur, a binary encounters multiple stars as it sinks through the nucleus toward the supermassive black hole. In this region, velocities are high, and interactions with stars can destroy binaries through ionization. We investigate wide ranges in initial mass function and internal energy of the binaries, and find that tidal separations, mergers, and ionizations are all likely outcomes for binaries near the galactic center. Tidally separated binaries will contribute to the LISA detection rate, and mergers will produce tens of events per year for Advanced LIGO. We show, therefore, that galactic nuclei are promising hosts of gravitational wave sources for both LISA and LIGO.