Chernoglazov, AlexanderHakobyan, HaykPhilippov, AlexanderPartial funding for Open Access provided by the UMD Libraries' Open Access Publishing Fund.We present the results of 3D particle-in-cell simulations that explore relativistic magnetic reconnection in pair plasma with strong synchrotron cooling and a small mass fraction of nonradiating ions. Our results demonstrate that the structure of the current sheet is highly sensitive to the dynamic efficiency of radiative cooling. Specifically, stronger cooling leads to more significant compression of the plasma and magnetic field within the plasmoids. We demonstrate that ions can be efficiently accelerated to energies exceeding the plasma magnetization parameter, ≫σ, and form a hard power-law energy distribution, fi ∝ γ−1. This conclusion implies a highly efficient proton acceleration in the magnetospheres of young pulsars. Conversely, the energies of pairs are limited to either σ in the strong cooling regime or the radiation burnoff limit, γsyn, when cooling is weak. We find that the high-energy radiation from pairs above the synchrotron burnoff limit, εc ≈ 16 MeV, is only efficiently produced in the strong cooling regime, γsyn < σ. In this regime, we find that the spectral cutoff scales as εcut ≈ εc(σ/γsyn) and the highest energy photons are beamed along the direction of the upstream magnetic field, consistent with the phenomenological models of gamma-ray emission from young pulsars. Furthermore, our results place constraints on the reconnection-driven models of gamma-ray flares in the Crab Nebula.en-USArticle